The
hydrogen evolution reaction (HER), as an efficient process
of converting various energies into high-purity hydrogen, has attracted
much attention from both scientific research studies and industrial
productions. However, its wide applications still confront considerable
difficulties, for example, bubble coverage on the electrode and bubble
dispersion in the electrolyte, which will disturb current distribution
and isolate active sites from reaction ions resulting in a high reaction
overpotential and large Ohmic voltage drop. Consequently, timely removing
the generated gas bubbles from the electrode as well as avoiding their
direct release into the electrolyte can be an effective approach to
address these issues. In this work, we have developed an elegant electrode,
that is, the integrated bundle electrode with wettability-gradient
copper cones, which is endowed with the multifunctions of continuous
generation, direct transport, and efficient collection of hydrogen
bubbles. All processes are proceeding on the electrode, which not
only remove the generated hydrogen bubbles efficiently but also prevent
the hydrogen bubbles from releasing into the electrolyte, which should
greatly advance the development of water electrolysis and offer inspirations
for people to fabricate more efficient HER devices.
Intravascular photoacoustic (IVPA) imaging technology enables the visualization of pathological characteristics (such as inflammation activities, lipid deposition) of the artery wall. Blood flushing is a necessary step in improving the imaging quality in in vivo IVPA imaging. But the limited imaging speed of the systems stretches their flushing time, which is an important obstacle of their clinical translations. In this paper, we report an improvement in IVPA/IVUS imaging speed to 100 frames per second. The high-speed imaging is demonstrated in rabbit in vivo, visualizing the nanoparticles accumulated on abdominal aorta wall at the wavelength of 1064 nm, in real time display. Blood flushing in vivo improves the IVPA signal-noise-ratio by around 3.5 dB. This study offers a stable, efficient and easy-to-use tool for instantaneous disease visualization and disease diagnosis in research and forwards IVPA/IVUS imaging technology towards clinical translations.
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