Spin-triplet superfluids can support exotic objects, such as half-quantum vortices characterized by the nontrivial winding of the spin structure. We present cantilever magnetometry measurements performed on mesoscopic samples of Sr(2)RuO(4), a spin-triplet superconductor. With micrometer-sized annular-shaped samples, we observed transitions between integer fluxoid states as well as a regime characterized by "half-integer transitions"--steps in the magnetization with half the height of the ones we observed between integer fluxoid states. These half-height steps are consistent with the existence of half-quantum vortices in superconducting Sr(2)RuO(4).
Photoemission and tunneling spectroscopies measure the energies at which single electrons can be added to or removed from an electronic system 1 . Features observed in such spectra have revealed electrons coupling to vibrational modes of ions both in solids 2 and in individual molecules 3 .Here we report the discovery of a sharp resonance in the tunneling spectrum of a 2D electron system. Its behavior suggests that it originates from vibrational modes, not involving ionic motion, but instead arising from vibrations of spatial ordering of the electrons themselves. In a twodimensional electronic system at very low temperatures and high magnetic fields, electrons can either condense into a variety of quantum Hall phases or arrange themselves into a highly ordered "Wigner" crystal lattice [4][5][6] . Such spatially ordered phases of electrons are often electrically insulating and delicate and have proven very challenging to probe with conventional methods.Using a unique pulsed tunneling method capable of probing electron tunneling into insulating phases, we observe a sharp peak with dependencies on energy and other parameters that fit to models for vibrations of a Wigner crystal 7,8 . The remarkable sharpness of the structure presents strong evidence of the existence of a Wigner crystal with long correlation length.Theory suggests that a Wigner crystal (WC) may exist near integer quantum Hall states as an insulating phase with expected transition temperature in the range of a few hundred millikelvin or below 5,6,[9][10][11][12] has proven difficult to demonstrate a long range ordered crystal; the observed features could arise from localization of electrons or a short-range ordered glassy phase. One method of detecting crystalline order is by means of observation of the crystal's vibrations. In prior measurements 1 , strong coupling of tunneling electrons to vibrational modes of ions have given rise to "bosonic peaks" in the tunneling spectra. Observation of such structure was essential to verifying the BCS theory of superconductivity 1 . In this letter, we report the first observation of a sharp peak in tunneling spectra that displays the characteristics of phonons of an electron crystal.As with a lattice formed by ions in normal materials, the WC has gapless phonon modes from transverse and longitudinal phonons. However, application of a magnetic field forces hybridizes the two modes into magnetoplasmon and magnetophonon modes 7,19 , with the magnetophonon mode remaining as a gapless Goldstone mode that signals the emergence of crystalline order (spontaneous translational symmetry breaking) 7,8 . A measurement revealing the sharp magnetophonon mode would constitute direct and conclusive evidence of the existence of the WC. In this study, we detect the presence of the magnetophonon spectrum through its modification of the tunneling density of states (TDOS), and we control the energy scale of the magnetophonon spectrum by tuning the electronic carrier density and applied magnetic field. Our measurements rely on a...
The single-particle spectral function measures the density of electronic states in a material as a function of both momentum and energy, providing central insights into strongly correlated electron phenomena. Here we demonstrate a high-resolution method for measuring the full momentum- and energy-resolved electronic spectral function of a two-dimensional (2D) electronic system embedded in a semiconductor. The technique remains operational in the presence of large externally applied magnetic fields and functions even for electronic systems with zero electrical conductivity or with zero electron density. Using the technique on a prototypical 2D system, a GaAs quantum well, we uncover signatures of many-body effects involving electron-phonon interactions, plasmons, polarons, and a phonon analog of the vacuum Rabi splitting in atomic systems.
We describe a feedback-based dynamic cantilever magnetometry technique capable of achieving thermal limited magnetic moment sensitivity with low applied fields. Using this technique, we have observed periodic entry of vortices into mesoscopic Sr2RuO4 rings. The quantized jump in the magnetic moment of the particle produced by individual vortices was measured with a resolution of 7×10−16 emu with an applied field of 1 Oe.
The development of robust computational protocols capable of accurately predicting the dielectric strengths of eco-friendly insulating gas candidates is crucial; however, it lacks relevant efforts significantly. Consequently, a series of computational protocols are employed in this study to enable the computational prediction of polarizability and ionization energy of eco-friendly, perfluorinated carbon-based candidates, followed by the equation-based prediction of their dielectric strength. The validation process associated with the prediction of the afore-mentioned variables for selected datasets confirms the suitability of the B3LYP-based prediction protocol for reproducing experimental values. Subsequently, the validation of dielectric strength prediction outlines the following three conclusions. (1) The referenced equation adopted from a previous study is incapable of predicting the dielectric strengths of 137 organic compounds present in our database. (2) Parameterization of the coefficients in the referenced equation leads to the accurate prediction of the dielectric strengths. (3) Incorporation of a novel variable, viz. molecular weight, into the referenced equation combined with the parameterization of the coefficients leads to a robust protocol capable of predicting dielectric strengths with high efficiencies even with a significantly smaller fitting dataset. This implies the development of a comprehensive solution capable of accurately predicting the dielectric strengths of a substantially large dataset.
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