Gold nanoparticles moving in aqueous solution under a optical vortex lattice are shown to present a complex collective optofluidic dynamics. Above a critical field intensity and concentration the system presents a spontaneous transition towards synchronised motion, driven by nonconservative optical forces, thermal fluctuations and hydrodynamic pairing. The system exhibits a rich assortment of collective dynamics such as strong unidirectional currents of nanoparticles at speeds of centimetres per second. This relatively simple optofluidic setup offers an alternative way to control mass and heat transport at the nanoscale, which has been so far elusive.
Superconducting films in contact with non-superconducting regular arrays can exhibit commensurability effects between the vortex lattice and the unit cell of the pinning array. These matching effects yield a slowdown of the vortex flow and the corresponding dissipation decrease. The superconducting samples are Nb films grown on Si substrates. We have studied these matching effects with the array on top, embedded or threading the Nb superconducting films and using different materials (Si, Cu, Ni, Py dots and dots fabricated with Co/Pd multilayers). These hybrids allow studying the contribution of different pinning potentials to the matching effects. The main findings are: i) Periodic roughness induced in the superconducting film is enough to generate resistivity minima; ii) A minor effect is achieved by magnetic pinning from periodic magnetic field potentials obtained by dots with out of plane magnetization grown on top of the superconducting film, iii) In the case of array of magnetic dots embedded in the films vortex flow probes the magnetic state; i.e. magnetoresistance measurements detect the magnetic state of very small nanomagnets. In addition, we have studied the role played by the local order in the commensurability effects. This was attained using an array that mimics a smectic crystal. We have found that preserving the local order is crucial. If the local order is not retained the magnetoresistance minima vanish.
The interaction forces between identical resonant molecules or nanoparticles, optically induced by a quasimonochromatic isotropic random light field, are theoretically analyzed. In general, the interaction force exhibits a far-field oscillatory behavior at separation distances larger than the light wavelength. However, we show that the oscillations disappear when the frequency of the random field is tuned to an absorption Fröhlich resonance, at which the real part of the particle's electric polarizability is zero. At the resonant condition, the interaction forces follow a long-range gravitylike inverse square distance law which holds for both near-and far-field separation distances.
The diffusion of a dimer made out of two resonant dipolar scatters in an optical lattice is theoretically analyzed. When a small particle diffuses through an optically induced potential landscape, its Brownian motion can be strongly suppressed by gradient forces, proportional to the particle's polarizability. For a single lossless monomer at resonance, the gradient force vanishes and the particle diffuses as in absence of external fields. However, we show that when two monomers link in a dimer, the multiple scattering among the monomers induces both a torque and a net force on the dimer's center of mass. This "self-induced back-action" force leads to an effective potential energy landscape, entirely dominated by the mutual interaction between monomers, which strongly influences the dynamics of the dimer. Under appropriate illumination, single monomers in a colloidal suspension freely diffuse while dimers become trapped. Our theoretical predictions are tested against extensive Langevin molecular dynamics simulations.
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