Tabletop coherent x-ray sources extending to multi-keV or higher photon energies have versatile applications, including in 4D imaging and semiconductor detectors. However, these sources can be realized only via high-order harmonic generation (HHG) with an ∼ 10 µ m laser interacting with neutral atoms. As shown in previous work by Popmintchev et al. [Science 350, 1225 (2015)10.1126/science.aac9755SCIEAS0036-8075], multiply ionized plasmas can efficiently produce hundred-eV harmonics with an ultraviolet laser. Here, we experimentally investigate multi-keV x-ray sources up to ∼ 5.2 k e V , the highest photon energy generated via HHG to date, to our knowledge, using a 1.45-µm driving laser that interacts with multivalent ions. Both the angular distribution and the ellipticity dependence of the signal are strong evidence of the HHG mechanism.

We demonstrate in this Letter the generation of carrier-envelope-phase (CEP)-stabilized laser pulses at 910 nm with simultaneously high-temporal-contrast, broad spectral bandwidths and few-cycle pulse durations. Through combining the techniques of cascaded optical parametric amplification (OPA) and second-harmonic generation (SHG) in the laser setup, a pulse temporal contrast as high as > 10 12 has been obtained at the laser output. During the OPA and SHG processes, both the pulse chirp and gain bandwidth are perfectly optimized, leading to the generation of 170 µJ pulses with > 200 n m bandwidth and ∼ 15 f s pulse duration. Moreover, the CEP of the laser is stabilized passively to a noise level of less than 340 mrad. This high-quality pulsed light source, as the seed laser of the deuterated potassium dihydrogen phosphate (DKDP)-based 100 PW system, will be integrated into the Station of Extreme Light facility in the near future.

A femtosecond mid-infrared optical vortex laser can be used for high harmonic generation to extend cutoff energy to the kilo-electron-volt range with orbital angular momentum, as well as other secondary radiations. For these, we demonstrate a high-energy femtosecond 4 μm optical vortex laser based on optical parametric chirped pulse amplification (OPCPA) for the first time. The optical vortex seed is generated from a femtosecond 4 μm laser by a silicon spiral phase plate with the topological charge l of 1 before the stretcher. Through using a two-stage collinear OPCPA amplifier, the chirped vortex pulse is amplified to 12.4 mJ with 200 nm full width at half-maximum bandwidth. After compression, the vortex laser pulse with 9.53 mJ, 119 fs can be obtained. Furthermore, the vortex characteristics of the laser beam are investigated and evaluated. This demonstration can scale to generate a higher-peak-power vortex mid-IR laser and pave a new way for high field physics.

The generation of high-peak-power, few-cycle mid-infrared (MIR) pulses using coherent beam combination and nonlinear pulse compression techniques simultaneously is demonstrated. The two pulses, with identical pulse energy of 2.8 mJ and pulse duration of 160 fs, are coherently combined at the input end of a krypton-filled hollow-core fiber (HCF), and then the bandwidth of the combined pulse is broadened to near an optical octave due to strong phase modulations, and the temporal width is compressed into a few-cycle regime. Finally, a 2.7 mJ, 22.9 fs, 20 Hz laser at 4 μm can be obtained, and the pulse peak power is greatly enhanced compared with that of conventional single-channel optical parametric chirped pulse-amplification systems. Furthermore, the peak power generated from this system has the prospect of further scaling up through use of more channels of coherent combination, which can pave a way to generate higher peak power ultra-intense MIR pulses for strong-field physics.