Abstract. Meridional atmospheric transport is an important process in the climate system and has implications for the availability of heat and moisture at high latitudes. Near-surface cold and warm temperature advection over the ocean in the context of extratropical cyclones additionally leads to important air–sea exchange. In this paper, we investigate the impact of these air–sea fluxes on the stable water isotope (SWI) composition of water vapour in the Southern Ocean's atmospheric boundary layer. SWIs serve as a tool to trace phase change processes involved in the atmospheric water cycle and, thus, provide important insight into moist atmospheric processes associated with extratropical cyclones. Here we combine a 3-month ship-based SWI measurement data set around Antarctica with a series of regional high-resolution numerical model simulations from the isotope-enabled numerical weather prediction model COSMOiso. We objectively identify atmospheric cold and warm temperature advection associated with the cold and warm sector of extratropical cyclones, respectively, based on the air–sea temperature difference applied to the measurement and the simulation data sets. A Lagrangian composite analysis of temperature advection based on the COSMOiso simulation data is compiled to identify the main processes affecting the observed variability of the isotopic signal in marine boundary layer water vapour in the region from 35 to 70∘ S. This analysis shows that the cold and warm sectors of extratropical cyclones are associated with contrasting SWI signals. Specifically, the measurements show that the median values of δ18O and δ2H in the atmospheric water vapour are 3.8 ‰ and 27.9 ‰ higher during warm than during cold advection. The median value of the second-order isotope variable deuterium excess d, which can be used as a measure of non-equilibrium processes during phase changes, is 6.4 ‰ lower during warm than during cold advection. These characteristic isotope signals during cold and warm advection reflect the opposite air–sea fluxes associated with these large-scale transport events. The trajectory-based analysis reveals that the SWI signals in the cold sector are mainly shaped by ocean evaporation. In the warm sector, the air masses experience a net loss of moisture due to dew deposition as they are advected over the relatively colder ocean, which leads to the observed low d. We show that additionally the formation of clouds and precipitation in moist adiabatically ascending warm air parcels can decrease d in boundary layer water vapour. These findings illustrate the highly variable isotopic composition in water vapour due to contrasting air–sea interactions during cold and warm advection, respectively, induced by the circulation associated with extratropical cyclones. SWIs can thus potentially be useful as tracers for meridional air advection and other characteristics associated with the dynamics of the storm tracks over interannual timescales.

Abstract. Meridional atmospheric transport is an important process in the climate system and has implications for the availability of heat and moisture at high latitudes. Near-surface advection of cold and warm temperature over the ocean in the context of extratropical cyclones additionally leads to important air–sea exchange. In this paper, we investigate the impact of these air–sea fluxes on the stable water isotope (SWI) composition of water vapour in the Southern Ocean’s atmospheric boundary layer. SWIs serve as a tool to trace phase change processes involved in the atmospheric water cycle and, thus, provide important insight into moist atmospheric processes associated with extratropical cyclones. Here we combine a three-month ship-based SWI measurement data set around Antarctica with a series of regional high resolution numerical model simulations from the isotope-enabled numerical weather prediction model COSMOiso. We objectively identify atmospheric cold and warm temperature advection associated with the cold and warm sector of extratropical cyclones, respectively, based on the air–sea temperature difference applied to the measurement and the simulation data sets. A Lagrangian composite analysis of cold and warm temperature advection based on the COSMOiso simulation data is compiled to identify the main processes affecting the observed variability of the isotopic signal in marine boundary layer water vapour in the region from 35° S to 70° S. This analysis shows that the cold and warm sectors of extratropical cyclones are associated with contrasting SWI signals. Specifically, the measurements show that the median values of δ18O and δ2H in the atmospheric water vapour are 3.6 ‰ and 23.2 ‰ higher during warm than during cold advection. The median value of the second-order isotope variable deuterium excess d, which can be used as a measure of non-equilibrium processes during phase changes, is 5.9 ‰ lower during warm than during cold advection. These characteristic isotope signals during cold and warm advection reflect the opposite air–sea fluxes associated with these large-scale transport events. The trajectory-based analysis reveals that the SWI signals in the cold sector are mainly shaped by ocean evaporation. In the warm sector, the air masses experience a net loss of moisture due to dew deposition as they are advected over the relatively colder ocean, which leads to the observed low d. We show that additionally the formation of clouds and precipitation in moist adiabatically ascending warm air parcels can decrease d in boundary layer water vapour. These findings illustrate the highly variable isotopic composition in water vapour due to contrasting air–sea interactions during cold and warm advection, respectively, induced by the circulation associated with extratropical cyclones. SWIs can thus potentially be useful as tracers for meridional air advection and other characteristics associated with the dynamics of the storm tracks over interannual timescales.

<p>Dynamical processes in the atmosphere strongly influence the large temporal and spatial variability of the atmospheric branch of the water cycle. For instance, the advection of air masses by synoptic-scale weather systems induces air-sea moisture fluxes such as evaporation, precipitation and dew deposition. It is important to better investigate and quantify this linkage between dynamical phenomena and details of the atmospheric water cycle. In addition, one of the big challenges in monitoring the atmospheric water cycle is the measurement of turbulent moisture fluxes over the ocean. Stable water isotopes (SWIs) serve as a tool to trace atmospheric processes which shape the atmospheric water cycle and, thus, provide important insights into moist processes associated with weather systems, in particular air-sea fluxes.</p><p>In this study, we investigate the impact of air-sea moisture fluxes on the variability of SWI signals in the marine boundary layer. Measurements of the second-order isotope variable deuterium excess in the marine boundary layer of the Southern Ocean show positive/negative anomalies in the cold/warm sector, respectively, of extra-tropical cyclone due to opposing moisture fluxes and non-equilibrium fractionation processes in the two sectors. The drivers of these contrasting SWI signals are analysed using the isotope-enabled Consortium for Small-Scale Modelling model for two case studies. The simulated isotope signals during the case studies show excellent agreement with ship-based isotope measurements from the Southern Ocean performed during the Antarctic Circumnavigation expedition in January and February 2017.</p><p>The main driver of SWI variability in the cold sector is enhanced ocean evaporation which substantially modifies the advected SWI signal from the Antarctic continent during a cold air outbreak. In the warm sector, dew deposition on the ocean surface and cloud formation are mainly driving the observed negative deuterium excess anomaly, which can be conserved and advected over several 100 km in the warm sector of an extratropical cyclone.</p><p>The results of this study illustrate the strong dependence of the isotopic composition of water vapour in the marine boundary layer on the predominant atmospheric large-scale flow situation. In particular in the storm track regions, the variability of SWIs in marine boundary layer water vapour is largely shaped by the sign and strength of air-sea fluxes induced by the meridional transport of air masses.</p>

Abstract. A substantial portion of the moisture transport into the Arctic occurs in episodic, high-amplitude events with strong impacts on the Arctic's climate system components such as sea ice. This study focuses on the origin of such moist-air intrusions during winter and examines the moisture sources, moisture transport pathways, and their linkage to the driving large-scale circulation patterns. For that purpose, 597 moist-air intrusions, defined as daily events of intense (exceeding the 90th anomaly percentile) zonal mean moisture transport into the polar cap (≥70∘ N), are identified. Kinematic backward trajectories combined with a Lagrangian moisture source diagnostic are then used to pinpoint the moisture sources and characterize the airstreams accomplishing the transport. The moisture source analyses show that the bulk of the moisture transported into the polar cap during these moist-air intrusions originates in the eastern North Atlantic with an uptake maximum poleward of 50∘ N. Trajectories further reveal an inverse relationship between moisture uptake latitude and the level at which moisture is injected into the polar cap, consistent with ascent of poleward-flowing air in a baroclinic atmosphere. Focusing on intrusions in the North Atlantic (424 intrusions), we find that lower tropospheric moisture transport is predominantly accomplished by two types of airstreams: (i) cold, polar air warmed and moistened by surface fluxes and (ii) air subsiding from the mid-troposphere into the boundary layer. Both airstreams contribute about 36 % each to the total transport. The former accounts for most of the moisture transport during intrusions associated with an anomalously high frequency of cyclones east of Greenland (218 intrusions), whereas the latter is more important in the presence of atmospheric blocking over Scandinavia and the Ural Mountains (145 events). Long-range moisture transport, accounting for 17 % of the total transport, dominates during intrusions with weak forcing by baroclinic weather systems (64 intrusions). Finally, mid-tropospheric moisture transport is invariably associated with (diabatically) ascending air and moisture origin in the central and western North Atlantic, including the Gulf Stream front, accounting for roughly 10 % of the total transport. In summary, our study shows that moist-air intrusions into the polar atmosphere result from a combination of airstreams with predominantly high-latitude or high-altitude origin, whose relative importance is determined by the underlying driving weather systems (i.e., cyclones and blocks).

Abstract. Poleward moisture transport occurs in episodic, high-amplitude events with strong impacts on the Arctic and its climate system components such as sea ice. This study focuses on the origin of such events and examines the moisture sources, moisture transport pathways, and their linkage to the large-scale circulation. For that purpose, 597 events of intense zonal mean poleward moisture transport at 70° N (exceeding the 90th anomaly percentile) are identified and kinematic backward trajectories from 70° N are computed to pinpoint the moisture sources and characterize the air-streams accomplishing the transport. The bulk of the moisture transported into the polar cap during these events originates in the eastern North Atlantic with an uptake maximum poleward of 50° N. This asymmetry between ocean basins is a direct consequence of the fact that most of the moisture transport into the polar cap occurs in this sector. As a result of the fairly high-latitude origin of the moisture, the median time moisture spends in the atmosphere prior to reaching 70° N amounts to about 2.5 days. Trajectories further reveal an inverse relationship between moisture uptake latitude and the level at which moisture is injected into the polar cap, consistent with ascent of poleward flowing air in a baroclinic atmosphere. Focusing on events for which 75 % of the zonal mean moisture transport takes place in the North Atlantic east of Greenland (424 events) reveals that lower tropospheric moisture transport results predominantly from two types of air-streams: (i) cold, polar air advected from the Canadian Arctic over the North Atlantic and around Greenland, whereby the air is warmed and moistened by surface fluxes, and (ii) air subsiding from the mid-troposphere into the boundary layer. Both air-streams contribute about 36 % each to the total transport. The former dominates the moisture transport during events associated with an anomalously high frequency of cyclones east of Greenland (218 events), whereas the latter is more important in the presence of atmospheric blocking over Scandinavia and the Ural (145 events). A substantial portion of the moisture sources associated with both types of air-streams are located between Iceland, the British Isles, and Norway. Long-range moisture transport, accounting for 17 % of the total transport, is the dominant type of air-stream during events with weak forcing by baroclinic weather systems (64 events). Finally, mid-tropospheric moisture transport is invariably associated with (diabatically) ascending air and moisture origin in the central and western North Atlantic, including the Gulf Stream front, accounting for roughly 10 % of the total transport. In summary, our study reveals that moisture injections into the polar atmosphere are not primarily caused by the poleward transport of warm and humid air from low latitudes – a conclusion that applies in particular to cases where the transport is driven by baroclinic weather systems such as extratropical cyclones. Instead, it results from a combination of air-streams with pre-dominantly high-latitude or high-altitude origin and their interplay with large-scale weather systems (e.g., cyclones, blocks).