The interdot correlation in a single pair of InAs∕GaAs barrier-coupled quantum dots (QDs) is investigated by microphotoluminescence spectroscopy, in which each QD is individually excited at unique energy levels. Surprisingly, we observe an anomalous increase in the luminescence intensity when the two QDs are excited simultaneously. This remarkable finding can be interpreted in terms of the electromagnetic coupling between QDs with thick barrier layers.

We propose and experimentally investigate an exciton molecule consisting of two different excitons in coupled quantum dots (QDs). Quantum mechanical coupling between double QDs leads to the creation of bonding and antibonding states and should yield an exciton molecule consisting of two excitons that originate from these two states. We prepared a quantum mechanically coupled QD system and succeeded in observing a single exciton molecule in a single pair of coupled QDs by means of a two-color excitation photoluminescence measurement.

We investigated the optical properties of an exciton and a charged exciton in an InAs/GaAs single quantum dot (QD) with truncated pyramidal shape by microspectroscopy, and clarified the difference of sub-band structure between the exciton and the charged exciton in the same single QD. We observed the exciton population of the excited states by monitoring the luminescence of the ground state exciton and succeeded in the experimental demonstration of Rabi oscillation of the exciton and the charged exciton. The transition dipole moments estimated from experimental results in a pure InAs QD are 32 and 40 D for the charged exciton and exciton, respectively, which were comparable to those in InGaAs QD.

We fabricated InAs/GaAs double quantum dot (QD) structures by molecular beam epitaxy (MBE) with the Indium-Flush method, where the energy separation between the electron levels of two QDs was less than the longitudinal optical (LO) phonon energy with a different barrier thickness. We confirm the peak energy shift between the double QDs in the photoluminescence (PL) spectra and assign this shift to the wave function coupling effect between the double dots. We also measured the time resolved PL spectra and observed the carrier transfer from smaller QDs to larger ones in the time domain. By estimating the tunneling time between double QDs, we obtain a tunneling time that is longer than the exciton decay time in single QD. Additionally, we mention the fade-out of the electron LO phonon interaction with the electron wave function coupling between double QDs based on the result of photoluminescence excitation measurements. These results suggest that our structures are attractive for quantum information processing.