Abstract-The interaction of laser radiation with single J aggregates of cyanine dyes is theoretically analyzed and numerically simulated. The quantum mechanical calculations of the equilibrium geometry and the ener gies and intensities of the lowest singlet electronic transitions in pseudoisocyanine chloride and its linear (chain) oligomers are fulfilled. The data of these calculations can serve as parameters of the analyzed model of interaction of J aggregates with radiation in the one particle density matrix approximation. This model takes into account relaxation processes, the annihilation of excitations at neighboring molecules, and inho mogeneous broadening. Assuming that the inhomogeneous broadening is absent, calculations demonstrate the existence of spatial bistability, molecular switching waves, and dissipative solitons. The effect of the inho mogeneous broadening and the radiation intensity on the effective coherence length in linear (chain) J aggre gates is analyzed.
Quantum fluctuations of two-dimensional dark dissipative solitons in an interferometer filled with a Kerr nonlinear medium are analyzed theoretically. The boundaries of the stability region of classical solitons excited in the considered interferometer by an external radiation are refined. The solution of the quantum problem is studied in the linear approximation. For this purpose, the formalism of expansion of the sought solution in discrete spectral functions is extended to the two-dimensional case. Using this expansion made it possible to construct a solution that describes fluctuations of collective variables of a two-dimensional soliton, namely, the coordinate of the center and momentum. Mean squares of quantum fluctuations of these quantities are calculated. Parameter domains in which there exist squeezed states of solitons with respect to each of the collective variables are determined. Comparative analysis of squeezing with respect to these variables for light and dark solitons is performed.
scite is a Brooklyn-based organization that helps researchers better discover and understand research articles through Smart Citations–citations that display the context of the citation and describe whether the article provides supporting or contrasting evidence. scite is used by students and researchers from around the world and is funded in part by the National Science Foundation and the National Institute on Drug Abuse of the National Institutes of Health.