The quantization of the electromagnetic field in a three-dimensional inhomogeneous dielectric medium with losses is carried out in the framework of a damped-polariton model with an arbitrary spatial dependence of its parameters. The equations of motion for the canonical variables are solved explicitly by means of Laplace transformations for both positive and negative time. The dielectric susceptibility and the quantum noise-current density are identified in terms of the dynamical variables and parameters of the model. The operators that diagonalize the Hamiltonian are found as linear combinations of the canonical variables, with coefficients depending on the electric susceptibility and the dielectric Green function. The complete time dependence of the electromagnetic field and of the dielectric polarization is determined. Our results provide a microscopic justification of the phenomenological quantization scheme for the electromagnetic field in inhomogeneous dielectrics.

The dynamics of a collection of resonant atoms embedded inside an inhomogeneous nondispersive and lossless dielectric is described with a dipole Hamiltonian that is based on a canonical quantization theory. The dielectric is described macroscopically by a position-dependent dielectric function and the atoms as microscopic harmonic oscillators. We identify and discuss the role of several types of Green tensors that describe the spatio-temporal propagation of field operators. After integrating out the atomic degrees of freedom, a multiple-scattering formalism emerges in which an exact Lippmann-Schwinger equation for the electric field operator plays a central role. The equation describes atoms as point sources and point scatterers for light. First, single-atom properties are calculated such as position-dependent spontaneous-emission rates as well as differential cross sections for elastic scattering and for resonance fluorescence. Secondly, multi-atom processes are studied. It is shown that the medium modifies both the resonant and the static parts of the dipoledipole interactions. These interatomic interactions may cause the atoms to scatter and emit light cooperatively. Unlike in free space, differences in position-dependent emission rates and radiative line shifts influence cooperative decay in the dielectric. As a generic example, it is shown that near a partially reflecting plane there is a sharp transition from two-atom superradiance to single-atom emission as the atomic positions are varied.

PACS. 42.50.Nn -Quantum optical phenomena in absorbing, dispersive and conducting media. PACS. 71.36.+c -Polaritons. PACS. 3.70.+k -Theory of quantized fields.Abstract. -The Hamiltonian of a polariton model for an inhomogeneous linear absorptive dielectric is diagonalized by means of Fano's diagonalization method. The creation and annihilation operators for the independent normal modes are explicitly found as linear combinations of the canonical operators. The coefficients in these combinations depend on the tensorial Green function that governs the propagation of electromagnetic waves through the dielectric. The time-dependent electromagnetic fields in the Heisenberg picture are given in terms of the diagonalizing operators. These results justify the phenomenological quantization of the electromagnetic field in an absorptive dielectric.c EDP Sciences