The addition of mixed double perovskite Ba2Y(Nb/Ta)O6 (BYNTO) to YBa2Cu3O7−δ (YBCO) thin films leads to a large improvement of the in-field current carrying capability. For low deposition rates, BYNTO grows as well-oriented, densely distributed nanocolumns. We achieved a pinning force density of 25 GN/m3 at 77 K at a matching field of 2.3 T, which is among the highest values reported for YBCO. The anisotropy of the critical current density shows a complex behavior whereby additional maxima are developed at field dependent angles. This is caused by a matching effect of the magnetic fields c-axis component. The exponent N of the current-voltage characteristics (inversely proportional to the creep rate S) allows the depinning mechanism to be determined. It changes from a double-kink excitation below the matching field to pinning-potential-determined creep above it.
Physical properties of a pyrohafnate compound Pr2Hf2O7 have been investigated by ac magnetic susceptibility χac(T ), dc magnetic susceptibility χ(T ), isothermal magnetization M (H) and heat capacity Cp(T ) measurements on polycrystalline as well as single crystal samples combined with high-resolution synchrotron x-ray diffraction (XRD) for structural characterization and inelastic neutron scattering (INS) to determine the crystal field energy level scheme and wave functions. Synchrotron XRD data confirm the ordered cubic pyrochlore (F d3m) structure without any noticeable site mixing or oxygen deficiency. No clear evidence of long range magnetic ordering is observed down to 90 mK, however the χac(T ) evinces slow spin dynamics revealed by a frequency dependent broad peak associated with spin freezing. The INS data reveal the expected five well defined magnetic excitations due to crystal field splitting of the J = 4 ground state multiplet of the Pr 3+ . The crystal field parameters and ground state wavefunction of Pr 3+ have been determined. The Ising anisotropic nature of magnetic ground state is inferred from the INS as well as χ(T ) and M (H) data. Together these properties make Pr2Hf2O7 a candidate compound for quantum spin-ice behavior.
There is growing evidence that the superconducting semimetal FeSe (Tc ∼ 8 K) is in the crossover regime between weak-coupling Bardeen-Cooper-Schrieffer (BCS) and strong-coupling Bose-Einsteincondensate (BEC) limits. We report on longitudinal and transverse thermal conductivities, κxx and κxy, respectively, in magnetic fields up to 20 T. The field dependences of κxx and κxy imply that a highly anisotropic small superconducting gap forms at the electron Fermi-surface pocket whereas a more isotropic and larger gap forms at the hole pocket. Below ∼ 1.0 K, both κxx and κxy exhibit distinct anomalies (kinks) at the upper critical field Hc2 and at a field H * slightly below Hc2. The analysis of the thermal Hall angle (κxy/κxx) indicates a change of the quasiparticle scattering rate at H * . These results provide strong support to the previous suggestion that above H * a distinct field-induced superconducting phase emerges with an unprecedented large spin imbalance.
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