We experimentally study the phase behavior of a charge-stabilized two-dimensional colloidal crystal which is subjected to a one-dimensional periodic light field. Such light fields are created by a scanned optical line tweezer which allows the variation of the periodicity without optical realignments. In order to realize a wide range of line spacings relative to the lattice constant, we use a suspension of silica particles in bromobenzene. This colloidal system has a Debye screening length of about 4.6 mm which results in the formation of crystals with lattice constants up to 20 mm. Because the refractive index of bromobenzene is larger than that of the colloids, optical gradient forces lead to the attraction of particles at regions where the intensity is smallest. Depending on the depth and periodicity of the optical potential, we observe the light-induced assembly of colloids into triangular, rhombic and square phases.
We experimentally study the phase behaviour of a charge-stabilized two-dimensional colloidal monolayer which is subjected to a one-dimensional quasiperiodic substrate potential. Upon increasing the laser intensity, we observe a transition from a periodic to a quasiperiodic state. It proceeds via the formation of an intermediate periodic average structure (PAS) which is related to the quasiperiodic lattice by a bounded 1 1 mapping. Because PAS can transform to crystals and quasicrystals by minute particle displacements, they provide a mechanism to allow for interesting insights into the relationship between periodic and quasiperiodic order.
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