We have generalized finite-difference (FD) simulations for time-dependent field propagation problems, in particular in view of ultra-short x-ray pulse propagation and dispersion. To this end, we first derive the stationary paraxial (parabolic) wave equation for the scalar field envelope in a more general manner than typically found in the literature. We then present an efficient FD implementation of propagators for different dimensionality for stationary field propagation, before we treat time-dependent problems by spectral decomposition, and suitable numerical sampling. We prove the validity of the numerical approach by comparison to analytical theory, using simple tractable propagation problems. Finally, we apply the framework to the problem of modal dispersion in X-ray waveguide. We show that X-ray waveguides can be considered as non-dispersive optical elements down to sub-femtosecond pulse width. Only when considering resonant absorption close to an X-ray absorption edge, we observe pronounced dispersion effects for experimentally achievable pulse widths. All code used for the work is made available as supplemental material.
We have coupled a nano-focused synchrotron beam into a planar x-ray waveguide structure through a thinned cladding, using the resonant beam coupling (RBC) geometry, which is well established for coupling of macroscopic x-ray beams into x-ray waveguides. By reducing the beam size and using specially designed waveguide structures with multiple guiding layers, we can observe two reflected beams of similar amplitudes upon resonant mode excitation. At the same time, the second reflected beam is shifted along the surface by several millimeters, constituting a exceptionally large Goos-Hänchen effect. We evidence this effect based on its characteristic far-field patterns resulting from interference of the multiple reflected beams. The experimental results are in perfect agreement with finite-difference simulations.
Iterative phase retrieval has been used to reconstruct the near-field distribution behind tailored X-ray waveguide arrays, by inversion of the measured far-field pattern recorded under fully coherent conditions. It is thereby shown that multi-waveguide interference can be exploited to control the near-field distribution behind the waveguide exit. This can, for example, serve to create a secondary quasi-focal spot outside the waveguide structure. For this proof of concept, an array of seven planar Ni/C waveguides are used, with precisely varied guiding layer thickness and cladding layer thickness, as fabricated by high-precision magnetron sputtering systems. The controlled thickness variations in the range of 0.2 nm results in a desired phase shift of the different waveguide beams. Two kinds of samples, a one-dimensional waveguide array and periodic waveguide multilayers, were fabricated, each consisting of seven C layers as guiding layers and eight Ni layers as cladding layers. These are shown to yield distinctly different near-field patterns.
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