This paper describes a method for aligning stiff, high-aspect-ratio microcrystals over macro-length scales using a polymer fiber drawing process. A composite preform was constructed with an interfacial, liquid shell layer of grapeseed oil suspending ytterbium-doped potassium lutetium fluoride microcrystals (30% Yb:K2LuF5, KLF) between adjacent cylindrical surfaces of acrylic (polymethyl methacrylate, PMMA). The mean length of synthesized KLF microcrystals was 67 microns, and the mean aspect ratio, equivalent to crystal length divided by diameter, was eight. The acrylic-host preform was drawn into fiber, resulting in uniform reduction of all cross-sectional dimensions by a factor of approximately 20 in the final fiber. A corresponding width reduction of the interstitial liquid-filled gap, containing microcrystals between the polymer surfaces, constrains the microcrystals and causes alignment of the crystal long axes parallel to the axis of the drawn composite fiber. Alignment was best for clearly separated microcrystals and improved even further with the longest lengths, or highest aspect-ratio microcrystals.