Due to the increasing demand for battery electric vehicles (BEVs), the need for vehicle battery raw materials is increasing. The traction battery (TB) of an electric vehicle, usually a lithium-ion battery (LIB), represents the largest share of a BEV’s CO2 footprint. To reduce this carbon footprint sustainably and to keep the raw materials within a closed loop economy, suitable and efficient recycling processes are essential. In this life cycle assessment (LCA), the ecological performance of a waterjet-based direct recycling process with minimal use of resources and energy is evaluated; only the recycling process is considered, waste treatment and credits for by-products are not part of the analysis. Primary data from a performing recycling company were mainly used for the modelling. The study concludes that the recycling of 1 kg of TB is associated with a global warming potential (GWP) of 158 g CO2 equivalents (CO2e). Mechanical removal using a water jet was identified as the main driver of the recycling process, followed by an air purification system. Compared to conventional hydro- or pyrometallurgical processes, this waterjet-based recycling process could be attributed an 8 to 26 times lower GWP. With 10% and 20% reuse of recyclate in new cells, the GWP of TBs could be reduced by 4% and 8%, respectively. It has been shown that this recycling approach can be classified as environmentally friendly.
Since environmental benefits and supply chain resilience are commonly assumed for circular economy strategies, this study tests this hypothesis in the context of lithium-ion battery recycling and cell manufacturing. Therefore, the use of recyclates from different cathode active materials and from different recycling routes, namely hydrometallurgy and direct recycling, in a subsequent cell production is modelled with the recyclate quotas prescribed by the amended European Battery Regulation and analysed using life cycle assessment methodology. This study concludes that both, negative and positive environmental impacts can be achieved by the usage of recyclates, depended on the cell technology and the recycling process chosen. Newly constructed lithium iron phosphate (LFP) cells using a share of 11.3% of recyclates, which are obtained from LFP cells by a hydrometallurgical process, achieve a deterioration in the ecology by 7.5% for the global warming potential (GWP) compared to LFP cells without any recyclate share at all. For the same recyclate quota scenario, hydrometallurgical recyclates from lithium nickel manganese cobalt oxide cells (NMC), on the other hand, achieve savings in GWP of up to 1.2%. Recyclates from direct recycling achieve savings in GWP for LPF and NMC of a maximum of 6.3% and 12.3%, by using a recyclate share of 20%. It can be seen that circular economy can raise large savings potentials ecologically, but can also have a contrary effect if not properly applied.
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