The recent severe and frequent PM2.5 (i.e., fine particles smaller than 2.5 µm) pollution in China has aroused unprecedented public concern. The first two years of PM2.5 measurements in China are reported and compared with those of Europe and the United States. The average PM2.5 concentration in China is approximately 5 times that over Europe and America. The contribution of atmospheric dispersion to such air quality is evaluated in this study. Air stagnation or its absence is a good indicator of the atmosphere’s capability to disperse its pollutants, but the NOAA definition of an air stagnation event is found to not be applicable to China since it depends on vertical mixing that is weakened in China by the effects of terrain. To address this deficiency, a new threshold for air stagnation events is proposed that depends on the 10-m wind speed, boundary layer height, and occurrence of precipitation. This newly defined air stagnation closely tracks the day-to-day variation of PM2.5 concentrations. Such events are more frequent over China than over Europe and the United States during autumn and winter, especially over the Sichuan basin and Jing-Jin-Ji region of China. If China had the same frequency of air stagnation as the United States or Europe, 67% and 82% of its stations would improve their current air quality during autumn and winter (e.g., an average of 12% decrease in PM2.5 concentrations for the Jing-Jin-Ji region in wintertime). Its severe pollution and frequent air stagnation conditions make controls on emission less effective in China than elsewhere.
[1] The Radiation Transfer Model Intercomparison (RAMI) initiative is a communitydriven exercise to benchmark the models of radiation transfer (RT) used to represent the reflectance of terrestrial surfaces. Systematic model intercomparisons started in 1999 as a self-organized, open-access, voluntary activity of the RT modeling community. The results of the first phase were published by Pinty et al. [2001]. The present paper describes the benchmarking protocol and the results achieved during the second phase, which took place during 2002. This second phase included two major components: The first one included a rerun of all direct-mode tests proposed during the first phase, to accommodate the evaluation of models that have been upgraded since, and the participation of new models into the entire exercise. The second component was designed to probe the performance of three-dimensional models in complex heterogeneous environments, which closely mimic the observations of actual space instruments operating at various spatial resolutions over forest canopy systems. Phases 1 and 2 of RAMI both confirm not only that a majority of the radiation transfer models participating in RAMI are in good agreement between themselves for relatively simple radiation transfer problems but also that these models exhibit significant discrepancies when considering more complex but nevertheless realistic geophysical scenarios. Specific recommendations are provided to guide the future of this benchmarking program (Phase 3 and beyond).
A rapid canopy reflectance model inversion experiment was performed using multi-angle reflectance data from the NASA Multi-angle Imaging Spectro-Radiometer (MISR) on the Earth Observing System Terra satellite, with the goal of obtaining measures of forest fractional crown cover, mean canopy height, and aboveground woody biomass for large parts of south-eastern Arizona and southern New Mexico (N200,000 km 2 ). MISR red band bidirectional reflectance estimates in nine views mapped to a 250 m grid were used to adjust the Simple Geometric-optical Model (SGM). The soil-understory background signal was partly decoupled a priori by developing regression relationships with the nadir camera blue, green, and nearinfrared reflectance data and the isotropic, geometric, and volume scattering kernel weights of the LiSparse-RossThin kernel-driven bidirectional reflectance distribution function (BRDF) model adjusted against MISR red band data. The SGM's mean crown radius and crown shape parameters were adjusted using the Praxis optimization algorithm, allowing retrieval of fractional crown cover and mean canopy height, and estimation of aboveground woody biomass by linear rescaling of the dot product of cover and height. Retrieved distributions of crown cover, mean canopy height, and aboveground woody biomass for forested areas showed good matches with maps from the United States Department of Agriculture (USDA) Forest Service, with R 2 values of 0.78, 0.69, and 0.81, and absolute mean errors of 0.10, 2.2 m, and 4.5 tons acre -1 (10.1 Mg ha -1 ), respectively, after filtering for high root mean square error (RMSE) on model fitting, the effects of topographic shading, and the removal of a small number of outliers. This is the first use of data from the MISR instrument to produce maps of crown cover, canopy height, and woody biomass over a large area by seeking to exploit the structural effects of canopies reflected in the observed anisotropy patterns in these explicitly multiangle data.
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