The discovery of two-dimensional magnets has initiated a new field of research, exploring both fundamental low-dimensional magnetism, and prospective spintronic applications. Recently, observations of magnetic skyrmions in the 2D ferromagnet Fe3GeTe2 (FGT) have been reported, introducing further application possibilities. However, controlling the exhibited magnetic state requires systematic knowledge of the history-dependence of the spin textures, which remains largely unexplored in 2D magnets. In this work, we utilise real-space imaging, and complementary simulations, to determine and explain the thickness-dependent magnetic phase diagrams of an exfoliated FGT flake, revealing a complex, history-dependent emergence of the uniformly magnetised, stripe domain and skyrmion states. The results show that the interplay of the dominant dipolar interaction and strongly temperature dependent out-of-plane anisotropy energy terms enables the selective stabilisation of all three states at zero field, and at a single temperature, while the Dzyaloshinksii-Moriya interaction must be present to realise the observed Néel-type domain walls. The findings open perspectives for 2D devices incorporating topological spin textures.
Topological charge plays a significant role in a range of physical systems. In particular, observations of real‐space topological objects in magnetic materials have been largely limited to skyrmions – states with a unitary topological charge. Recently, more exotic states with varying topology, such as antiskyrmions, merons, or bimerons and 3D states such as skyrmion strings, chiral bobbers, and hopfions, have been experimentally reported. Along these lines, the realization of states with higher‐order topology has the potential to open new avenues of research in topological magnetism and its spintronic applications. Here, real‐space imaging of such spin textures, including skyrmion, skyrmionium, skyrmion bag, and skyrmion sack states, observed in exfoliated flakes of the van der Waals magnet Fe3−xGeTe2 (FGT) is reported. These composite skyrmions may emerge from seeded, loop‐like states condensed into the stripe domain structure, demonstrating the possibility to realize spin textures with arbitrary integer topological charge within exfoliated flakes of 2D magnets. The general nature of the formation mechanism motivates the search for composite skyrmion states in both well‐known and new magnetic materials, which may yet reveal an even richer spectrum of higher‐order topological objects.
The ability to dope transition metal dichalcogenides such as tungsten diselenide (WSe2) with magnetic transition metal atoms in a controlled manner has motivated intense research with the aim of generating dilute magnetic semiconductors. In this work, semiconducting WSe2 monolayers, substitutionally doped with vanadium atoms, are investigated using low‐temperature luminescence and optoelectronic spectroscopy. V‐dopants lead to a p‐type doping character and an impurity‐related emission ≈160 meV below the neutral exciton, both of which scale with the nominal percentage of V‐dopants. Measurements using field‐effect devices of 0.3% V‐doped WSe2 demonstrate bipolar carrier tunability. The doped monolayers display a clear magnetic hysteresis in transport measurements both under illumination and without illumination, whereas the valley polarization of the excitons reveals a nonlinear g‐factor without a magnetic hysteresis within the experimental uncertainty. Hence, this work on V‐doped WSe2 provides crucial insights concerning suitable characterization methods on magnetic properties of doped 2D materials.
van der Waals heterostructures made from graphene and three-dimensional topological insulators promise very high electron mobilities, a nontrivial spin texture, and a gate-tunability of electronic properties. Such a combination of advantageous electronic characteristics can only be achieved through proximity effects in heterostructures, as graphene lacks a large enough spin–orbit interaction. In turn, the heterostructures are promising candidates for all-electrical control of proximity-induced spin phenomena. Here, we explore epitaxially grown interfaces between graphene and the lattice-matched topological insulator Bi2Te2Se. For this heterostructure, spin–orbit coupling proximity has been predicted to impart an anisotropic and electronically tunable spin texture. Polarization-resolved second-harmonic generation, Raman spectroscopy, and time-resolved magneto-optic Kerr microscopy are combined to demonstrate that the atomic interfaces align in a commensurate symmetry with characteristic interlayer vibrations. By polarization-resolved photocurrent measurements, we find a circular photogalvanic effect which is drastically enhanced at the Dirac point of the proximitized graphene. We attribute the peculiar gate-tunability to the proximity-induced interfacial spin structure, which could be exploited for, e.g., spin filters.
The dynamics of fluxons in long Josephson junctions is a well-known example of soliton physics and allows for studying highly nonlinear relativistic electrodynamics on a microscopic scale. Such fluxons are supercurrent vortices that can be accelerated by bias current up to the Swihart velocity, which is the characteristic velocity of electromagnetic waves in the junction. We experimentally demonstrate slowing down relativistic fluxons in Josephson junctions whose bulk superconducting electrodes are replaced by thin films of a high kinetic inductance superconductor. Here, the amount of magnetic flux carried by each supercurrent vortex is significantly smaller than the magnetic flux quantum [Formula: see text]. Our data show that the Swihart velocity is reduced by about one order of magnitude compared to conventional long Josephson junctions. At the same time, the characteristic impedance is increased by an order of magnitude, which makes these junctions suitable for a variety of applications in superconducting electronics.
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