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Coal macrolithotypes control the reservoir heterogeneity, which plays a significant role in the exploration and development of coalbed methane. Traditional methods for coal macrolithotype evaluation often rely on core observation, but these techniques are non-economical and insufficient. The geophysical logging data are easily available for coalbed methane exploration; thus, it is necessary to find a relationship between core observation results and wireline logging data, and then to provide a new method to quantify coal macrolithotypes of a whole coal seam. In this study, we propose a L-Index model by combing the multiple geophysical logging data with principal component analysis, and we use the L-Index model to quantitatively evaluate the vertical and regional distributions of the macrolithotypes of No. 3 coal seam in Zhengzhuang field, southern Qinshui basin. Moreover, we also proposed a S-Index model to quantitatively evaluate the general brightness of a whole coal seam: the increase of the S-Index from 1 to 3.7, indicates decreasing brightness, i.e., from bright coal to dull coal. Finally, we discussed the relationship between S-Index and the hydro-fracturing effect. It was found that the coal seam with low S-Index values can easily form long extending fractures during hydraulic fracturing. Therefore, the lower S-Index values indicate much more favorable gas production potential in the Zhengzhuang field. This study provides a new methodology to evaluate coal macrolithotypes by using geophysical logging data.