By coupling femtosecond pulses at lambda - 1.55mum in a short length (Z - 95 cm) of photonic crystal fiber, we observe the simultaneous generation of two visible radiation components. Frequency-resolved optical gating experiments combined with analysis and modal simulations suggest that the mechanism for their generation is third-harmonic conversion of the fundamental pulse and its split Raman self-shifted component.

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Using experimental feedback, we demonstrate that a chirped-pulse amplifier can adaptively learn to compensate for the higher-order phase dispersion that is inherent in the amplification process. A genetic algorithm-based search routine is used to repetitively update the pulse phase in a programmable pulse stretcher during a plasma breakdown experiment to maximize the magnitude of spectral blueshift. Reductions in pulse duration from 37 to 30 fs and substantially better wing structure are typically obtained as a result of the optimization.

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