We have performed inelastic neutron scattering on a single crystal sample of Sr 14 Cu 24 O 41 to study the spin dynamics of the Cu 2 O 3 spin ladder layers, and CuO 2 chains. Data collected with incident energies of 50 meV, 200 meV, 350 meV and 500 meV are best fitted with a dispersion with a spin gap of 32.5±0.1 meV and a maximum of 193.5±2.4 meV, consistent with a coupling along the ladders, J || = 130 meV and a rung coupling J ⊥ =72 meV. We find that excitations with an energy transfer of approximately 11.5 meV can be described solely in terms of a dimer chain with an antiferromagnetic intra-dimer coupling, J 1 = 11.2 meV, between next-nearest-neighbour Cu ions and a ferromagnetic inter-dimer coupling, J 2 = -1.1 meV. The dimers are separated by two Cu ions providing a periodicity for the dimer chain of five units.
We report significant intergrain magnetoresistance (IMR) in polycrystalline double perovskites of SrFe1−x(Mo or Re)xO3 at room temperature. Systematics of the temperature dependence of IMR indicates that the observed large room-temperature IMR in SrFe1/2Mo1/2O3 originates from the ferrimagnetic nature of insulating grain boundaries as well as the half-metallicity of this perovskite. Our results indicate that a new avenue for spin-polarized tunneling junctions is to utilize insulating interface layers with ferromagnetic or ferrimagnetic coupling.
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