We demonstrate a nanostructure layer made of Ni80Fe20 (permalloy:Py) thin film conjugated MoS2 nano-flakes. Layers are made based on a single-step co-deposition of Py and MoS2 from a single solution where ionic Ni and Fe and MoS2 flakes co-exist. Synthesized thin films with MoS2 flakes show increasing coercivity and enhancement in magneto-optical Kerr effect. Ferromagnetic resonance linewidth as well as the damping parameter increaseed significantly compared to that of the Py layer due to the presence of MoS2. Raman spectroscopy and elemental mapping is used to show the quality of MoS2 within the Py thin film. Our synthesis method promises new opportunities for electrochemical production of functional spintronic-based devices.