Chemical transport associated with the dynamics of the Asian summer monsoon (ASM) system is investigated using model output from the National Center for Atmospheric Research (NCAR) Whole Atmosphere Community Climate Model run in specified dynamics mode. The 3‐D day‐to‐day behavior of modeled carbon monoxide is analyzed together with dynamical fields and transport boundaries to identify preferred locations of uplifting from the boundary layer, the role of subseasonal‐scale dynamics in the upper troposphere and lower stratosphere (UTLS), and the relationship of ASM transport and the stratospheric residual circulation. The model simulation of CO shows the intraseasonal east‐west oscillation of the anticyclone may play an essential role in transporting convectively pumped boundary layer pollutants in the UTLS. A statistical analysis of 11 year CO also shows that the southern flank of the Tibetan plateau is a preferred location for boundary layer tracers to be lofted to the tropopause region. The vertical structure of a model tracer (E90) further shows that the rapid ASM vertical transport is only effective up to the tropopause level (around 400 K). The efficiency of continued vertical transport into the deep stratosphere is limited by the slow ascent associated with the zonal‐mean residual circulation in the lower stratosphere during northern summer. Quasi‐isentropic transport near the 400 K potential temperature level is likely the most effective process for ASM anticyclone air to enter the stratosphere.

Most chemistry-climate models show an intensification of the Brewer-Dobson circulation (BDC) in the stratosphere associated with increasing greenhouse gas emissions and ozone depletion in the last decades, but this trend remains to be confirmed in observational data. In this work the evolution of the advective BDC for the period 1979-2012 is evaluated and compared in three modern reanalyses (ERA-Interim, MERRA, and JRA-55). Three different estimates of the BDC are computed for each reanalysis, one based on the definition of the residual circulation and two indirect estimates derived from momentum and thermodynamic balances. The comparison among the nine estimates shows substantial uncertainty in the mean magnitude (∼40%) but significant common variability. The tropical upwelling series show variability linked to the stratospheric quasi-biennial oscillation and to El Niño-Southern Oscillation (ENSO) and also reflect extreme events such as major sudden stratospheric warmings and volcanic eruptions. The trend analysis suggests a strengthening of tropical upwelling of around 2-5%/decade throughout the layer 100-10 hPa. The global spatial structure of the BDC trends provides evidence of an overall acceleration of the circulation in both hemispheres, with qualitative agreement among the estimates. The global BDC trends are mainly linked to changes in the boreal winter season and can be tracked to long-term increases in the resolved wave drag in both hemispheres.

It is an outstanding issue to what degree trends in stratospheric mean age of air reflect changes in the (slow) residual circulation and how they are affected by (fast) eddy mixing. We present a method to quantify the effects of mixing and residual circulation on mean age trends, based on simulations with the Chemical Lagrangian Model of the Stratosphere (CLaMS) driven by ERA‐Interim reanalysis and on the integrated tracer continuity equation. During 1990–2013, mean age decreases throughout most of the stratosphere, qualitatively consistent with results based on climate model simulations. During 2002–2012, age changes show a clear hemispheric asymmetry in agreement with satellite observations. We find that changes in the residual circulation transit time cannot explain the mean age trends, and including the integrated effect of mixing is crucial. Above about 550 K (about 22 km), trends in the mixing effect on mean age appear to be coupled to residual circulation changes.