We report on the implementation of a time-multiplexed click detection scheme to probe quantum correlations between different spatial optical modes. We demonstrate that such measurement setups can uncover nonclassical correlations in multimode light fields even if the single mode reductions are purely classical. The nonclassical character of correlated photon pairs, generated by a parametric down-conversion, is immediately measurable employing the theory of click counting instead of low-intensity approximations with photoelectric detection models. The analysis is based on second- and higher-order moments, which are directly retrieved from the measured click statistics, for relatively high mean photon numbers. No data postprocessing is required to demonstrate the effects of interest with high significance, despite low efficiencies and experimental imperfections. Our approach shows that such novel detection schemes are a reliable and robust way to characterize quantum-correlated light fields for practical applications in quantum communications.

We provide a rigorous treatment of the entanglement properties of two-mode Gaussian states in atmospheric channels by deriving and analyzing the input-output relations for the corresponding entanglement test. A key feature of such turbulent channels is a non-trivial dependence of the transmitted continuous-variable entanglement on coherent displacements of the quantum state of the input field. Remarkably, this allows one to optimize the entanglement certification by modifying local coherent amplitudes using a finite, but optimal amount of squeezing. In addition, we propose a protocol which, in principle, renders it possible to transfer the Gaussian entanglement through any turbulent channel over arbitrary distances. Therefore, our approach provides the theoretical foundation for advanced applications of Gaussian entanglement in free-space quantum communication.

Quantum metrology and quantum information necessitate a profound study of suitable states. Attenuations induced by free-space communication links or fluctuations in the generation of such states limit the quantum enhancement in possible applications. For this reason we investigate quantum features of mixtures of so-called N00N states propagating in atmospheric channels. First, we show that noisy N00N states can still yield a phase resolution beyond classical limitations. Second, we identify entanglement of noisy N00N states after propagation in fluctuating loss channels. To do so, we apply the partial transposition criterion. Our theoretical analysis formulates explicit bounds which are indispensable for experimental verification of quantum entanglement and applications in quantum metrology.

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