We performed simultaneous, multispectral CRDS measurements that for the first time use the Supercontinuum light source. We called this approach Supercontinuum Cavity Ring-Down Spectrography (SC CRDSpectrography) and successfully applied it to measuring the absorption spectrum of NO2 gas at a concentration of 2 ppm. The extrapolated sensitivity of our setup was much greater, about 5 ppb. The ppb sensitivity level is comparable to this obtainable with single wavelength dye-lasers based CRDS systems. It is, therefore, feasible to construct extremely broadband and sensitive CRDS devices basing on the SC CRDSpectrography scheme.
We show experimentally that the interaction of two multifilamenting beams in fused silica with incidence angles up to a few degrees results in an increase in the symmetry of the continuum emission from D 2 to C ϱ around the axis of symmetry between the two beams. We observe an intense white disk between the locations of the individual conical emission patterns, reducing the conical emission in each of them. We attribute this behavior to an enhanced self-phase modulation in the interference region between the two beams. This frequency conversion depletes by more than 40% the energy initially available in the photon bath to feed filaments.
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