A split-and-delay unit for the extreme ultraviolet and soft X-ray spectral regions has been built which enables time-resolved experiments at beamlines FL23 and FL24 at the Free-electron LASer in Hamburg (FLASH). Geometric wavefront splitting at a sharp edge of a beam splitting mirror is applied to split the incoming soft X-ray pulse into two beams. Ni and Pt coatings at grazing incidence angles have been chosen in order to cover the whole spectral range of FLASH2 and beyond, up to hν = 1800 eV. In the variable beam path with a grazing incidence angle of ϑd = 1.8°, the total transmission (T) ranges are of the order of 0.48 < T < 0.84 for hν < 100 eV and T > 0.50 for 100 eV < hν < 650 eV with the Ni coating, and T > 0.06 for hν < 1800 eV for the Pt coating. For a fixed beam path with a grazing incidence angle of ϑf = 1.3°, a transmission of T > 0.61 with the Ni coating and T > 0.23 with a Pt coating is achieved. Soft X-ray pump/soft X-ray probe experiments are possible within a delay range of −5 ps < Δt < +18 ps with a nominal time resolution of t r = 66 as and a measured timing jitter of t j = 121 ± 2 as. First experiments with the split-and-delay unit determined the averaged coherence time of FLASH2 to be τc = 1.75 fs at λ = 8 nm, measured at a purposely reduced coherence of the free-electron laser.

The pulse duration in short-pulse schemes for Self-Amplified Spontaneous Emission Free Electron Lasers (SASE FELs) is limited by the FEL coherence time. A recently proposed concept allows to overcome the coherence time barrier and to obtain much shorter pulses. When the lasing part of an electron bunch is much shorter than the coherence time, one can suppress the radiation in the long main undulator while preserving microbunching within that short lasing slice. Then, a short radiation pulse is produced in a relatively short radiator. A possible suppression method, an excessive reverse undulator taper, is discussed and illustrated numerically in this paper. We also performed the first experimental tests of this method at the soft X-ray FEL user facility FLASH. The measured pulse duration approaches 1 fs (FWHM) at the wavelength of 5 nm.

We present the temporal characteristics of the split-and-delay unit at FLASH2 via visibility measurements which characterize the temporal resolution of the combined system of the FEL and the split-and-delay unit. The use of the splitand-delay unit at FLASH2 allows the users at the beamlines FL23 and FL24 at DESY to perform such pump-probe experiments. By using wavefront beam splitting, grazing incidence mirrors, and two different coatings the whole spectral region of FLASH2 is covered, and even harmonics up to 1800 eV are transmitted with a transmission of T > 0.06. It is concluded that user experiments with a pump-probe scheme from the picosecond regime down into the sub-femtosecond region can be carried out.

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The pulse duration in short-pulse schemes for Self-Amplified Spontaneous Emission Free Electron Lasers (SASE FELs) is limited by the FEL coherence time. A recently proposed concept allows to overcome the coherence time barrier and to get much shorter pulses. When the lasing part of an electron bunch is much shorter than the coherence time, one can suppress the radiation in the long main undulator while preserving microbunching within that short lasing slice. Then a short radiation pulse is produced in a relatively short radiator. A possible suppression method, an excessive reverse undulator taper, is discussed and illustrated numerically in this paper. We also performed first experimental tests of this method at the soft X-ray FEL user facility FLASH. The measured pulse duration approaches 1 fs (FWHM) at the wavelength of 5 nm.