We report on a 2ω-OPSL-pumped passively Q-switched Pr:LiYF laser operating at the wavelengths of 523, 607, and 640 nm. For this, we utilized a Co-doped MgAlO (MALO) crystal as a saturable absorber in the visible range for the first time, to the best of our knowledge. In the green spectral region, the pulse duration was 210 ns with a pulse energy of 3.6 μJ and a repetition rate of 125 kHz. The minimum pulse duration of 87 ns at the highest pulse energy of 8.6 μJ was obtained at a repetition rate of 110 kHz at 607 nm. The highest Q-switched average laser power of 1.4 W was obtained at an absorbed continuous-wave pump power of 3.3 W with a slope efficiency of 47% at 640 nm. Absorption saturation measurements with Co:MALO were performed, and ground and excited state absorption cross sections in the visible spectral range were determined.

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An investigation of Tm-Ho energy transfer in Tm(5at.%),Ho(0.4at.%):KYW single crystal by two independent techiques was performed. Based on fluorescence dynamics measurements, energy transfer parameters P 71 and P 28 for direct (Tm→Ho) and back (Ho→Tm) transfers, respectively, as well as equilibrium constant Θ were evaluated. The obtained results were supported by calculation of microscopic interaction parameters according to the Förster-Dexter theory for a dipoledipole interaction. Diode-pumped continuous-wave operation of Tm,Ho:KYW microchip laser was demonstrated, for the first time to our knowledge. Maximum output power of 77 mW at 2070 nm was achieved at the fundamental TEM 00 mode.

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