High-contrast, intense single-cycle pulses are highly desirable tools in ultrafast science, enabling highest temporal resolution, pushing matter to extreme conditions, and serving as drivers in petahertz electronics. In this Letter, we use thin solid plates in a double multi-plate supercontinuum configuration, delivering a broadband spectrum spanning from ∼ 400 to ∼ 1000 n m at the − 20 d B intensity level to produce a single-cycle pulse. We show that the spectral broadening by self-phase modulation with few-cycle pulses is more suitable for compression than the single-cycle limit than with multi-cycle pulses. The pulses are compressed to 2.6 fs pulses, close to the transform limit of 2.55 fs, with an energy of 0.235 mJ. They exhibit an excellent power stability of 0.5% rms over 3 h and a beam profile. The obtained single-cycle pulses can be utilized in many applications, such as generation of isolated attosecond pulses via high-order harmonic generation, investigation of ultrafast phenomena with extreme temporal resolution, or high-intensity laser-solid experiments.

Dynamic control of material properties using strong-field, narrowband THz sources has drawn attention because it allows selective manipulation of quantum states on demand by coherent excitation of specific low-energy modes in solids. Yet, the lack of powerful narrowband lasers with frequencies in the range of a few to a few tens of THz has restricted the exploration of hidden states in condensed matter. Here, we report the optimization of an optical parametric amplifier (OPA) and the efficient generation of a strong, narrowband THz field. The OPA has a total conversion efficiency of > 55%, which is the highest value reported to date, with an excellent energy-stability of 0.7% RMS over 3 h. We found that the injection of a high-energy signal beam to a power amplification stage in an OPA leads to high-efficiency and a super-Gaussian profile. By difference-frequency generation of two chirped OPA signal pulses in an organic nonlinear crystal, we obtained a THz pulse with an energy of 3.2 μJ, a bandwidth of 0.5 THz, and a pulse duration of 860 fs tunable between the 4 and 19 THz regions. This corresponds to an internal THz conversion efficiency of 0.4% and a THz field strength of 6.7 MV/cm. This approach demonstrates an effective way to generate narrow-bandwidth, intense THz fields.

No abstract