[1] We demonstrate first measurements of the aerosol indirect effect using ground-based remote sensors at a continental US site. The response of nonprecipitating, icefree clouds to changes in aerosol loading is quantified in terms of a relative change in cloud-drop effective radius for a relative change in aerosol extinction under conditions of equivalent cloud liquid water path. This is done in a single column of air at a temporal resolution of 20 s (spatial resolution of $100 m). Cloud-drop effective radius is derived from a cloud radar and microwave radiometer. Aerosol extinction is measured below cloud base by a Raman lidar. Results suggest that aerosols associated with maritime or northerly air trajectories tend to have a stronger effect on clouds than aerosols associated with northwesterly trajectories that also have local influence. There is good correlation (0.67) between the cloud response and a measure of cloud turbulence.

[1] The contribution of coastal oceans to the global air-sea CO 2 flux is poorly quantified due to insufficient availability of observations and inherent variability of physical, biological and chemical processes. We present simulated air-sea CO 2 fluxes from a high-resolution biogeochemical model for the North American east coast continental shelves, a region characterized by significant sediment denitrification. Decreased availability of fixed nitrogen due to denitrification reduces primary production and incorporation of inorganic carbon into organic matter, which leads to an increase in seawater pCO 2 , but also increases alkalinity, which leads to an opposing decrease in seawater pCO 2 . Comparison of simulations with different numerical treatments of denitrification and alkalinity allow us to separate and quantify the contributions of sediment denitrification to air-sea CO 2 flux. The effective alkalinity flux resulting from denitrification is large compared to estimates of anthropogenically driven coastal acidification.

Energetic constraints on precipitation are useful for understanding the response of the hydrological cycle to ongoing climate change, its response to possible geoengineering schemes, and the limits on precipitation in very warm climates of the past. Much recent progress has been made in quantifying the different forcings and feedbacks on precipitation and in understanding how the transient responses of precipitation and temperature might differ qualitatively. Here, we introduce the basic ideas and review recent progress. We also examine the extent to which energetic constraints on precipitation may be viewed as radiative constraints and the extent to which they are confirmed by available observations. Challenges remain, including the need to better demonstrate the link between energetics and precipitation in observations and to better understand energetic constraints on precipitation at sub-global length scales.

Arctic amplification (AA)—referring to the enhancement of near-surface air temperature change over the Arctic relative to lower latitudes—is a prominent feature of climate change with important impacts on human and natural systems. In this review, we synthesize current understanding of the underlying physical mechanisms that can give rise to AA. These mechanisms include both local feedbacks and changes in poleward energy transport. Temperature and sea ice-related feedbacks are especially important for AA, since they are significantly more positive over the Arctic than at lower latitudes. Changes in energy transport by the atmosphere and ocean can also contribute to AA. These energy transport changes are tightly coupled with local feedbacks, and thus their respective contributions to AA should not be considered in isolation. It is here emphasized that the feedbacks and energy transport changes that give rise to AA are sensitively dependent on the state of the climate system itself. This implies that changes in the climate state will lead to changes in the strength of AA, with implications for past and future climate change.