Monte Carlo computer simulations confirmed that an increase in density has a minor effect on the weakening of neutron transport and, therefore, the optimum composition of a shielding concrete against gamma radiation is different than the one against neutron radiation. Neutron radiation shielding is a two-step process: slowing down of fast neutrons and absorption of thermal ones. Both result from the atomic composition of the barrier but their dependence on specified atomic compositions and moisture content is different. The aim of the presented research is to develop a high density concrete the composition of which would also assure good efficiency of neutron shielding. Neutron transport through standard cement mortar, PCC mortar, normal-weight concrete and magnetite heavy-weight concrete has been analyzed in the paper. The goal in research was to find an influence of the cement type, polymer addition, density and moisture content on the shielding properties against neutron. The research based on convergent results of MC computer simulations and real experiments confirmed the influence of the cement type on fast neutron attenuation. It was also found that each 1% of moisture content makes 10% increase of fast neutron thermalization effectiveness, what is a little less than it was estimated for cement based mortars. It was also proved that heavyweight concrete is not proper solution for shielding against fast neutrons, but its efficiency is visible in the case of thermal neutrons absorption, probably due to increase of Fe content at the expense of Si and O in the atomic composition as well as water retained by magnetite aggregate.
Concrete has been used as a shield against high-energy photons (gamma) and neutrons since the beginning of use of nuclear reaction in energy, medicine and research. State of knowledge in shielding concrete technology is that while in case of protection against gamma radiation an increase in density caused by change of aggregate type for heavy-weight one is usually an efficient solution, the protection against neutrons is more complex. It is due to the differences in interactions of neutrons with the matter, depending on their kinetic energy and cross-sections for different reactions of the component atoms of the cement paste and the aggregate. The paper presents the results of the project NGS-Concrete - New-Generation Shielding Concrete. The aim is to design the composition of concrete against ionizing radiation, achieved by the use of experiment based on multi-criteria optimization of materials supported by the Monte Carlo simulations. Better concrete is the one that absorbs more thermal neutrons and slows down more fast neutrons at the same time. In the paper both results of Monte Carlo simulations and experimental studies on ordinary and heavyweight concrete containing epoxy polymer additive are presented. Close values of thermal neutron attenuation coefficients proved good accordance between simulation and experiment. The final conclusion is that epoxy resin is an efficient additive for neutron shielding concretes improving its ability to protect mainly against low energy neutrons. In experimental measurement there has not been observed an improvement of fast neutron attenuation due to increase of hydrogen atom content introduced with epoxy.
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