Striving to improve the critical current density Jc of superconducting YBa2Cu3O6+x (YBCO) thin films via enhanced vortex pinning, the interplay between film growth mechanisms and the formation of nanosized defects, both natural and artificial, is systematically studied in undoped and BaZrO3 (BZO)-doped YBCO thin films. The films were grown via pulsed laser deposition (PLD), varying the crystal grain size of the targets in addition to the dopant content. The microstructure of the PLD target has been observed to have a great impact on that of the deposited thin films, including the formation of vortex pinning centers, which has direct implications on the superconducting performance, especially on the isotropy of flux pinning properties. Based on experimentally measured angular dependencies of Jc, coupled with a molecular dynamics (MD) simulation of flux pinning in the YBCO films, we present a quantitative model of how the splay and fragmentation of BZO nanorods artifically introduced into the YBCO film matrix explain the majority of the observed critical current anisotropy.
In order to understand how the doping with self-assembled nanorods of different sizes and concentrations as well as applied magnetic fields affect the critical current anisotropy in YBa 2 cu 3 o 7−x (YBCO) thin films close to YBCO c-axis, we present an extensive and systematic computational study done by molecular dynamics simulation. the simulations are also used to understand experimentally measured J c (θ) curves for BaHfO 3 , BaZrO 3 and BaSno 3 doped YBCO thin films with the help of nanorod parameters obtained from transmission electron microscopy measurements. our simulations reveal that the relation between applied and matching field plays a crucial role in the formation of J c (θ)-peak around YBCO c-axis (c-peak) due to vortex-vortex interactions. We also find how different concentrations of different size nanorods effect the shape of the c-peak and explain how different features, such as double c-peak structures, arise. In addition to this, we have quantitatively explained that, even in an ideal superconductor, the overdoping of nanorods results in decrease of the critical current. our results can be widely used to understand and predict the critical current anisotropy of YBco thin films to improve and develop new pinscapes for various transport applications.High temperature superconductors (HTS) are expected to have large number of applications in different fields of technology and power industry in the future 1-3 . Since all known HTS are of type II, the critical current passed through them is highly dependent on the surrounding magnetic field due to the movement of vortices. Thus, to enhance and widen the usability of HTS, the dynamics of vortices need to be well understood.Among the high temperature superconductors, YBa 2 Cu 3 O 7−x (YBCO) seems the most practical choice when thinking for the applications 1 . The intrinsic anisotropy of the critical current, in thin films and coated conductors, can be modified by adding impurities within the lattice of YBCO which pin the vortices restricting their movement. Based on growth conditions and lattice mismatch between the YBCO and the dopant as well as their elastic properties 4,5 , impurities such as Y 2 O 3 6 , BaCeO 3 7-9 and BaZrO 3 (BZO) 10,11 can form uncorrelated randomly distributed nanoparticles within the YBCO lattice. Under optimized deposition conditions, via a spontaneous phase-separation and strain-driven self-assembly process during film deposition 12 , self-assembly of nanorods of BaHfO 3 (BHO) 1 , BaZrO 3 (BZO) 4,13,14 , BaSnO 3 (BSO) 15,16 , Ba 2 YTaO 3 (BYTO) 17 or Ba 2 YNbO 6 (BYNO) 18 within the YBCO lattice can be realized.Recently, a topic of interest has been to add both point-like nanodots and nanorods within the YBCO lattice simultaneously. This has been achieved by doping YBCO simultaneously with both BYTO and BYNO (referred as BYNTO) with an additional rare earth oxide, leading to continuous niobiate/tantalate nanorods and rare-earth oxide nanoparticles 19 . A lot of experimental research has been done in order to understand the...
A molecular dynamics (MD) simulation to simulate the vortices in superconductors with artificial pinning sites is presented. The simulation reproduces the correct anisotropic behavior in angular dependence of critical current. We also show that the shape of the [Formula: see text] curve depends on the size of the pinning sites and the change from p = 0.5 to [Formula: see text] is due to the breaking of the vortex lattice to individually acting vortices. The results beautifully correspond to experimental data. Furthermore, we found that the size and shape of the c-axis peak observed with columnar pinning sites in [Formula: see text] also depends on the size of the rods, larger pinning sites leading to wider peaks. The results obtained from the MD-simulation are similar to those of the much more computationally intensive Ginzburg-Landau simulations. Furthermore, the MD-simulations can provide insight to the vortex dynamics within the samples.
The flux pinning properties of the high temperature superconductor YBa2Cu3O7−δ (YBCO) have been conventionally improved by creating both columnar and dot-like pinning centres into the YBCO matrix. To study the effects of differently doped multilayer structures on pinning, several samples consisting of a multiple number of individually BaZrO3 (BZO) and BaCeO3 (BCO) doped YBCO layers were fabricated. In the YBCO matrix, BZO forms columnar and BCO dot-like defects. The multilayer structure improves pinning capability throughout the whole angular range, giving rise to a high critical current density, J c. However, the BZO doped monolayer reference still has the most isotropic J c. Even though BZO forms nanorods, in this work the samples with multiple thin layers do not exhibit a c axis peak in the angular dependence of J c. The angular dependencies and the approximately correct magnitude of J c were also verified using a molecular dynamics simulation.
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