The Technical Design for the COMET Phase-I experiment is presented in this paper. COMET is an experiment at J-PARC, Japan, which will search for neutrinoless conversion of muons into electrons in the field of an aluminum nucleus ($\mu$–$e$ conversion, $\mu^{-}N \rightarrow e^{-}N$); a lepton flavor-violating process. The experimental sensitivity goal for this process in the Phase-I experiment is $3.1\times10^{-15}$, or 90% upper limit of a branching ratio of $7\times 10^{-15}$, which is a factor of 100 improvement over the existing limit. The expected number of background events is 0.032. To achieve the target sensitivity and background level, the 3.2 kW 8 GeV proton beam from J-PARC will be used. Two types of detectors, CyDet and StrECAL, will be used for detecting the $\mu$–$e$ conversion events, and for measuring the beam-related background events in view of the Phase-II experiment, respectively. Results from simulation on signal and background estimations are also described.
Advances in electron and probe microscopies allow 10 pm or higher precision in measurements of atomic positions. This level of fidelity is sufficient to correlate the length (and hence energy) of bonds, as well as bond angles to functional properties of materials. Traditionally, this relied on mapping locally measured parameters to macroscopic variables, for example, average unit cell. This description effectively ignores the information contained in the microscopic degrees of freedom available in a high-resolution image. Here we introduce an approach for local analysis of material structure based on statistical analysis of individual atomic neighbourhoods. Clustering and multivariate algorithms such as principal component analysis explore the connectivity of lattice and bond structure, as well as identify minute structural distortions, thus allowing for chemical description and identification of phases. This analysis lays the framework for building image genomes and structure–property libraries, based on conjoining structural and spectral realms through local atomic behaviour.
Advances in high resolution imaging and scanning transmission electron microscopies as well as probe-based microscopies, extend beyond simple visualization of atomic structure of matter by allowing high (10 pm or better) precision measurements of atomic positions. Such a high level of fidelity is sufficient to correlate the length and hence energy of individual bonds, as well as bond angles to functional properties of materials. We introduce an algorithm for local analysis of material structure based on the statistical analysis of individualized, local atomic neighborhoods. Our clustering analysis explores the connectivity of lattice, allowing for efficient chemical description and identification of phases and structural defects in multiphase samples. This analysis lays the framework for building image genomes and structure-property libraries, based on conjoining structural and spectral realms through local atomic behavior.Algorithms like k-means clustering on multi-phase regions allow identification of minute structural distortions, providing framework for description of local physical functionalities. As a model system, we have chosen mixed oxide Mo-V-M-O (M = Nb, Ta, Te and/or Sb), which is currently the most promising catalyst for many industrially important reactions, such as propane (amm)oxidation.[1] Our algorithm yields absolute positions of each atom in an image, as well as local descriptors such as column intensity and peak width determined at the refinement stage. Significant improvements in atom finding based on target defined search are made over the traditional peak fitting methods. [2, 3] Atom tilts as well as correction approaches based on the recovered image data are explored. [4].The number of nearest neighbors, or the search radius, can be defined separately and are chosen depending on the type analysis. In the simplest case neighbors are chosen based on dominate symmetry, e.g. 6 for hexagonal lattice, or 4/8 for cubic lattice. Once the local neighborhood is established, the clustering algorithm is utilized with an appropriate selection metric of interest to sort the local neighborhoods. Shown in Figure 1(a) is a raw image of Mo-V-M-O mixed MA and M2 phases. We have specified 6 neighbors as well as 6 clusters; the results of a distance to neighbor based metric are shown in Figure 1(b) and a 4 cluster angle to neighbor based metric in Figure 1(c). Rotation is accounted for by always placing the first neighbor atom in the same location relative to the center and filling the rest in a clockwise fashion. The analysis clearly distinguishes different areas of the image based on the similarity of chemical neighborhoods of their constituent atoms, whose role and effects are discussed in detail. Figure 1(d) is a FFT of the overall image shown in Fig. 1(a), panels (e) and (f) show average atomic neighborhoods for 6 and 50 neighbors respectively. Figure 1(g) is a clustering dendrogram for the distance to neighbor case used to define the final number of clusters. We believe this approach paves the way for...
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