Novel magnetic titanium dioxide nanoparticles decorated with methyltrimethoxysilane (Fe 3 O 4 @TiO 2 -MTMOS) were successfully fabricated via a sol-gel method at room temperature. The synthesized material was characterized using Fourier transform infrared spectroscopy, X-ray diffraction, scanning electron microscopy, energy-dispersive X-ray spectroscopy, thermogravimetric analysis and vibrating sample magnetometry. The removal efficiency of the adsorbent was evaluated through the adsorption of methylene blue (MB) dye from water samples. The adsorption isotherm and kinetics were evaluated using various models. The Langmuir model indicated a high adsorption capacity (11.5 mg g −1 ) of Fe 3 O 4 @TiO 2 -MTMOS. The nanocomposite exhibited high removal efficiency (96%) and good regeneration (10 times) compared to Fe 3 O 4 and Fe 3 O 4 @TiO 2 at pH = 9.0. Based on the adsorption mechanism, electrostatic interaction plays a main role in adsorption since MB dye is cationic in nature at pH = 9, whereas the adsorbent acquired an anionic nature. The newly synthesized Fe 3 O 4 @TiO 2 -MTMOS can be used as a promising material for efficient removal of MB dye from aqueous media.KEYWORDS adsorption isotherm and kinetics, Fe 3 O 4 @TiO 2 nanoparticles, Fe 3 O 4 @TiO 2 -methyltrimethoxysilane nanocomposite, methylene blue dye

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