Topological insulators are a striking example of materials in which topological invariants are manifested in robustness against perturbations [1,2]. Their most prominent feature is the emergence of topological edge states with reduced dimension at the boundary between areas with distinct topological invariants. The observable physical effect is unidirectional robust transport, unaffected by defects or disorder. Topological insulators were originally observed in the integer quantum Hall effect [3], and subsequently suggested [4-6] and observed [7] even in the absence of magnetic field. These were fermionic systems of correlated electrons. However, during the past decade the concepts of topological physics have been introduced into numerous fields beyond condensed matter, ranging from microwaves [8,9] and photonic systems [10-12] to cold atoms [13,14], acoustics [15,16] and even mechanics [17,18]. Recently, topological insulators were proposed [19-21] in exciton-polariton systems organized as honeycomb (graphene-like) lattices, under the influence of a magnetic field. Topological phenomena in polaritons are fundamentally different from all topological effects demonstrated experimentally thus far: exciton-polaritons are part-light part-matter quasiparticles emerging from the strong coupling of quantum well excitons and cavity photons [22]. Here, we demonstrate experimentally the first exciton-polariton topological insulator. This constitutes the first symbiotic light-matter topological insulators. Our polariton lattice is excited non-resonantly, and the chiral topological polariton edge mode is populated by a polariton condensation mechanism. We use scanning imaging techniques in real-space and in Fourier-space to measure photoluminescence, and demonstrate that the topological edge mode avoids defects, and that the propagation direction of the mode can be reversed by inverting the applied magnetic field. Our exciton-polariton topological insulator paves the way for a variety of new topological phenomena, as they involve light-matter interaction, gain, and perhaps most importantly -exciton-polaritons interact with one another as a nonlinear many-body system.Microcavity exciton-polaritons (polaritons) are composite bosons originating from the strong coupling of quantum well excitons to microcavity photons. While the excitonic fraction provides a strong non-linearity, the photonic part results in a low effective mass, allowing the formation of a driven-dissipative Bose-Einstein condensate [23,24] and a superfluid phase [25], making polaritons being referred to as "quantum fluids of light" [26]. For the epitaxially well-controlled III-V semiconductor material system, a variety of techniques are available to micropattern such cavities in order to precisely engineer the potential landscapes of polaritons [27]. With the recent advances of bringing topological effects to the realms of photonics [8][9][10][11][12]28], several avenues to realize topological edge propagation with polaritons have been suggested [19][20][21], wi...
Unlike radiowave antennas, so far optical nanoantennas cannot be fed by electrical generators. Instead, they are driven by light 1 or indirectly via excited discrete states in active materials 2,3 in their vicinity. Here we demonstrate the direct electrical driving of an in-plane optical antenna by the broadband quantum-shot noise of electrons tunnelling across its feed gap. The spectrum of the emitted photons is determined by the antenna geometry and can be tuned via the applied voltage. Moreover, the direction and polarization of the light emission are controlled by the antenna resonance, which also improves the external quantum efficiency by up to two orders of magnitude. The one-material planar design offers facile integration of electrical and optical circuits and thus represents a new paradigm for interfacing electrons and photons at the nanometre scale, for example for on-chip wireless communication and highly configurable electrically driven subwavelength photon sources.Radio-and microwaves can be generated by currents that oscillate within antennas driven by high-frequency voltage sources that extend up into the 100 GHz regime. Sources for optical and infrared radiation are traditionally based on transitions between quantum states or bulky thermal sources because conventional electrical circuits are unable to generate oscillating currents with frequencies in the high terahertz regime 4 . As a result, the well-developed and powerful concepts of antenna theory are difficult to apply to optical radiation, the opposite of Feynman's anticipation 5 . However, in 1976 it was already shown that visible light can be generated through electron tunnelling in large-area vertically stacked metal-insulator-metal (MIM) junctions 6 . Soon after, it was proposed theoretically that such light emission is caused by quantum-shot noise that results in broadband current fluctuations, a picture that was recently proved conclusively 7,8 . Theoretical considerations suggest that quantum yields of up to 10% may be achieved using this mechanism 9,10 . However, experimental observations of light emission using scanning tunnelling microscopy typically yield much lower efficiencies 11-13 .Here we exploit quantum-shot noise to generate optical-frequency current oscillations within an in-plane antenna gap and thus create, for the first time, an electrically driven optical antenna. We show that coupling to a well-defined radiative antenna mode increases the efficiency of light emission by two orders of magnitude and provides full control over the properties of the emitted photons. As the optical antenna and tunnelling device are fully integrated, additional functionalities, such as gate electrodes, gap modifications and additional passive or active elements, may easily be incorporated. Furthermore, ultrafast amplitude and frequency modulation can be achieved.To realize an electrically driven optical antenna the challenge is to implement a lateral tunnel junction in the feed gap of an electrically connected optical antenna on an insulati...
2The interaction of light and matter, i.e. absorption and emission of photons, can be considerably enhanced in the presence of strongly localized and therefore highly intense optical near fields 1 .Plasmonic antennas consisting of pairs of closely spaced metal nano particles have gained much attention in this context since they provide the possibility to strongly concentrate optical fields into the gap between the two metal particles [2][3][4] . Pairs of closely spaced metal nanoparticles supporting plasmonic gap resonances consequently find broad applications, e.g. in single-emitter surfaceenhanced spectroscopy 5,6 , quantum optics 7 , extreme nonlinear optics 8-10 , optical trapping 11 , metamaterials 12, 13 and molecular opto-electronics 14 .The success of metal-insulator-metal structures is based on two fundamental properties of their anti-symmetric electromagnetic gap modes. (i) As a direct consequence of the boundary conditions, the dominating field components normal to the metal-dielectric interfaces are sizable only inside the dielectric gap. This means that for anti-symmetric gap modes the achievable field confinement is not limited by the skin depth of the metal, but is solely determined by the actual size of the gap. (ii) Since the free electrons of the metal respond resonantly to an external optical frequency field, enormous surface charge accumulations, accompanied by ultra-intense optical near fields, will occur. In addition, with decreasing gap width, stronger attractive coulomb forces 4 across the gap lead to further surface-charge accumulation and a concomitantly increased near-field intensity enhancement. We therefore conclude that an experimental realization of atomic-scale concentration of electromagnetic fields at visible frequencies is possible but it requires atomic-scale shape control of the field-confining structure, i.e. the gap, as well as a careful assignment and selection of suitable optical modes.Here we achieve atomic-scale confinement of electromagnetic fields at visible frequencies by combining for the first time both atomic-scale shape control of the field confining structure 15 as well as a careful selection and assignment of suitable optical modes [16][17][18] . We study single-crystalline nanorods which self-assemble into side-by-side aligned dimers with gap widths below 0.5 nm. Sideby-side aligned nanorod dimers possess various distinguishable symmetric and anti-symmetric 3 modes in the visible range 19 . In contrast to previous work 20-22 we demonstrate full control over symmetric and anti-symmetric optical modes by means of white-light scattering experiments. We experimentally demonstrate the presence of atomic-scale light confinement in these structures by observing an extreme > 800 meV hybridization splitting of corresponding symmetric and antisymmetric dimer modes. Our results open new perspectives for atomically-resolved spectroscopic imaging, deeply nonlinear optics and attosecond physics, cavity optomechanics and ultra-sensing as well as quantum optics.To obtain nano...
Atomic monolayers of transition metal dichalcogenides represent an emerging material platform for the implementation of ultra compact quantum light emitters via strain engineering. In this framework, we discuss experimental results on creation of strain induced single photon sources using a WSe 2 monolayer on a silver substrate, coated with a very thin dielectric layer. We identify quantum emitters which are formed at various locations in the sample. The emission is highly linearly polarized, stable in linewidth and decay times down to 100 ps are observed. We provide numerical calculations of our monolayer-metal device platform to assess the strength of the radiative decay 1 rate enhancement by the presence of the plasmonic structure. We believe, that our results represent a crucial step towards the ultra-compact integration of high performance single photon sources in nanoplasmonic devices and circuits.Single photon sources are considered as a key building block for quantum networks, quantum communications and optical quantum information processing. 15 To fully harness the properties of such non-classical light sources, core requirements include their long-term stability, 6,7 brightness 811 and scalability in the fabrication process. Recently, quantum light emission from inorganic two dimensional layers of transition metal dichalcogenides (TMDC) 1216 has been demonstrated. While the nanoscopic origin of tight exciton localization is still to be explored, engineering the morphology of carrier substrates and thus the strain eld in the monolayers 17 has enabled position control over such quantum emitters. 1820 One outstanding problem, which we address in this report, is the emission enhancement of such quantum emitters in atomic monolayers. The layered nature of the materials and their intrinsic robustness with regard to open surfaces (due to absence of dangling bonds) naturally puts plasmonic approaches in the focus of interest. A single dipole emitter close to a plasmonic nanoparticle, which act as an optical antenna, 21,22 experience a modied photonic mode density, leading to enhanced radiative decay rates and thus a spontaneous emission enhancement. The enhanced intensity results from an amplied electric eld intensity due to localized surface plasmon resonance of metal nanoparticles. 18,23,24 Plasmonic tuning of the optical properties of molecules, such as dyes close to a metal surface is a topic which is subject to investigations since the 1980s. Pronounced coupling phenomena of dye molecules with surface plasmon resonances in ultra-thin silver lms has been shown via luminescence and absorption studies, 25 as well as resonant transmission. 26 Enhanced uorescence of molecules coupled to Ag-islands has been studied in, 27 whereas uorescence quenching of dye molecules or colloidal CdSe quantum dots in the closest vicinity of metallic surfaces has also been identied to act signicantly on the emitters' decay dynamics. 28,29 Hence it is important to separate the emitters from the metallic layers via a non-conduct...
Yagi-Uda antennas are a key technology for efficiently transmitting information from point to point using radio waves. Since higher frequencies allow higher bandwidths and smaller footprints, a strong incentive exists to shrink Yagi-Uda antennas down to the optical regime. Here we demonstrate electrically-driven Yagi-Uda antennas for light with wavelength-scale footprints that exhibit large directionalities with forward-to-backward ratios of up to 9.1 dB. Light generation is achieved via antenna-enhanced inelastic tunneling of electrons over the antenna feed gap. We obtain reproducible tunnel gaps by means of feedback-controlled dielectrophoresis, which precisely places single surface-passivated gold nanoparticles in the antenna gap. The resulting antennas perform equivalent to radio-frequency antennas and combined with waveguiding layers even outperform RF designs. This work paves the way for optical on-chip data communication that is not restricted by Joule heating but also for advanced light management in nanoscale sensing and metrology as well as light emitting devices.
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