Specific very dry high-ozone layers, starting roughly two days after the onset of high-pressure periods during the warm season, have been reproducibly observed in the middle and upper troposphere with the ozone lidar in Garmisch-Partenkirchen (Germany). These episodes, previously not understood, were recently analysed based on extending backward simulations with the FLEXPART particle dispersion model to as many as twenty days and on jet-stream analyses including calculations with the LAGRANTO transport model. In all six cases analysed the model results indicate ozone import from the stratosphere on an extremely long path along the subtropical jet stream over the Pacific Ocean, Asia and, in part, all the way back to the Atlantic Ocean. The analysis suggests that stratospheric influence is the most important factor for the increase in ozone and is related to rather shallow transfer of air from the stratosphere into the upper- and mid-tropospheric air streams observed with the lidar. Contributions from the boundary layers of East Asia and North America are just occasionally present, in one case documented by a very dense aerosol plume from the Asian deserts. The considerable vertical and temporal extent of many of these layers and peak ozone mixing ratios between 80 and 150 ppb suggest that the observations are related to an important mechanism for stratosphere-to-troposphere transport (STT) and also confirm the model predictions of pronounced and persistent STT along the subtropical jet stream
Abstract. Very dry high-ozone layers have been repeatedly observed with the ozone lidar in Garmisch-Partenkirchen (Germany) starting one or two days after the onset of high-pressure periods during the warm season. These episodes have been analysed by trajectory calculations and extended simulations with the FLEXPART particle dispersion model. Mixed contributions from the stratosphere over the Pacific Ocean and the boundary layers of East Asia and North America were found. The stratospheric influence is mostly dominating and caused by a rather shallow transfer from the stratosphere into these rapid upper- and mid-tropospheric air streams. The considerable vertical extent of these layers and peak ozone mixing ratios between 80 and 150 ppb suggest an important mechanism for stratosphere-to-troposphere transport.
Specific very dry high-ozone layers have been repeatedly observed in the middle and upper troposphere with the ozone lidar in Garmisch-Partenkirchen (Germany), starting roughly two days after the onset of high-pressure periods during the warm season. These episodes, previously not understood, were recently analysed based on extended simulations with the FLEXPART particle dispersion model and jet-stream analyses with the LAGRANTO transport model. The model results indicate import from the stratosphere along the subtropical jet stream over the Pacific Ocean and all the way back to the Atlantic Ocean, in some cases mixed with stratospheric air from intrusions over the North-West Pacific Ocean. Occasionally, also air from the boundary layers of East Asia and North America was admixed. The analysis suggests that stratospheric influence is the most important factor for the increase in ozone and is related to a rather shallow transfer of air from the stratosphere into the rapid upper-and mid-tropospheric air streams observed with the lidar. The in part considerable vertical and temporal extent of these layers and peak ozone mixing ratios between 80 and 150 unit{ppb} suggest this to be an important mechanism for stratosphere-to-troposphere transport
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