We take advantage of nonlinear properties associated with chi(3) tensor elements in BaF2 cubic crystal to improve the temporal contrast of femtosecond laser pulses. The technique presented is based on cross-polarized wave (XPW) generation. We have obtained a transmission efficiency of 10% and 10(-10) contrast with an input pulse in the millijoule range. This filter does not affect the spectral shape or the phase of the cleaned pulse. It also acts as an efficient spatial filter. In this method the contrast enhancement is limited only by the extinction ratio of the polarization discrimination device.

Nonlinear polarization rotation and generation of a polarization component orthogonal to the input beam were observed along fourfold axes of YVO 4 and BaF 2 crystals. We demonstrate experimentally that in both crystals the angle of rotation is proportional, at low intensities, to the square of the product of the input intensity and the crystal length and is the result of simultaneous action of two third-order processes. This type of nonlinear polarization rotation is driven by the real part of the cubic susceptibility. The recorded energy exchange between the two orthogonal components can exceed 10%. It is to our knowledge the highest energy-conversion efficiency achieved in a single beam nonresonant (3) interaction. A simple theoretical model is elaborated to describe the dependence of nonlinear polarization rotation and orthogonal polarization generation on the intensity of the input beam at both low-and high-intensity levels. It reveals the potential contributions from the real and the imaginary parts of the susceptibility tensor. Moreover, this kind of measurement is designed to permit the determination of the magnitude and the sign of the anisotropy of the real part of third-order nonlinearity in crystals with cubic or tetragonal symmetry on the basis of polarization-rotation measurements. The xxxx (3) component of the third-order susceptibility tensor and its anisotropy sign and amplitude value for BaF 2 and YVO 4 crystals are estimated and discussed.

International audienceWe present an experimental demonstration of a renewed set up, with respect to the one described in [A. Jullien et al, Opt. Lett. 30, 920 (2005)], that enables more reliable and robust performances in the increase of the contrast ratio (CR) of energetic femtosecond pulses. The new approach is based on the use of two successive crystals situated at optimum position that generate cross polarized waves whose individual effect interferes constructively. This arrangement overcomes the limitation of the single crystal schemes for temporal cleaning – the early saturation of the transmission efficiency, previously observed when either using a relatively thick crystal or increasing intensities up to its damage threshold. A theoretical model that predicts the output CR is developed for the first time. It shows that the CR depends on the initial CR and the extinction ratio of the polarizers used. The measured temporal CR 10^-10 is in accordance with theoretical predictions

International audienceCross-polarized wave (XPW) generation is used for the contrast improvement of ultra-intense femtosecond laser pulses in a double CPA configuration. We present theoretical and experimental evidence that the XPW output spectrum depends in a predictable way on the input chirp. Therefore, a chirp controlled pulse can experience a pulse duration shortening up to a factor of sqrt(3), and an initial amount of chirp that leads to the exact preservation of the spectral width of a given pulse can be predicted

We propose a highly efficient scheme for temporal filters devoted to femtosecond pulse contrast enhancement. The filter is based on cross-polarized wave generation with a spatially suger-Gaussian-shaped beam. In a single nonlinear crystal scheme the energy conversion to the cross-polarized pulse can reach 28%. We demonstrate that the process enables a significant spectral broadening. For an efficiency of 23% the pulse shortening is estimated to 2.2, leading to an intensity transmission of the nonlinear filter of 50%.