The first stage of the petawatt excimer laser project started at the P.N. Lebedev Physical Institute, implements a development of multiterawatt hybrid GARPUN-MTW laser facility for generation of ultra-high intensity subpicosecond ultraviolet (UV) laser pulses. Under this project, a multi-stage e-beam-pumped 100-J, 100-ns GARPUN KrF laser was upgraded with a femtosecond Ti:Sapphire front-end, to produce combined subpicosecond/nanosecond laser pulses with variable time delay. Attractive possibility to amplify simultaneously short and long pulses in the same large-scale KrF amplifiers is analyzed with regard to the fast-ignition, inertial confinement fusion problem. Detailed description of hybrid laser system is presented with synchronized KrF and Ti:Sapphire master oscillators. Based on gain and absorption measurements at GARPUN amplifier and numerical simulations with a quasi-stationary code, we are predicting that 1.6 J can be obtained in a short pulse at hybrid GARPUN-MTW Ti:Sapphire/KrF laser facility, combined with several tens of joules in nanosecond pulse. Amplified spontaneous emission, which is responsible for the pre-pulse formation on a target, was also investigated: its acceptable level can be provided by properly choosing staged gain or loading the amplifiers by quasi-steady laser radiation. Fluorescence and transient absorption spectra of Ar/Kr/F 2 mixtures conventionally used in KrF amplifiers were recorded to find out the possibility for femtosecond pulse amplification at the broadband Kr 2 F (4 2 G ! 1,2 2 G) transition, which benefits in 100 times higher saturation energy density than for KrF (B ! X) transition.
A technique using the broadband emission of a laser plume as probe radiation is applied to record UV-visible (190-510 nm) absorption spectra of Ne, Ar, and Kr, pure and in binary mixtures under moderate e-beam excitation up to 1 MW/cm(3). In all the rare gases and mixtures, the absorption spectra show continuum related to Rg(2) (+) homonuclear ions [peaking at λ∼285, 295, and 320 nm in Ne, Ar, and Kr(Ar/Kr), respectively] and a number of atomic lines related mainly to Rg(∗)(ms) levels, where m is the lowest principal quantum number of the valence electron. In argon, a continuum related to Ar(2) (∗) (λ∼325 nm) is also recorded. There are also trains of narrow bands corresponding to Rg(2) (∗)(npπ (3)Π(g))←Rg(2) (∗)(msσ (3)Σ(u) (+)) transitions. All the spectral features mentioned above were reported in literature but have never been observed simultaneously. Although charge transfer to a homonuclear ion of the heavier additive is commonly believed to dominate in binary rare-gas mixtures, it is found in this study that in Ne/Kr mixture, the charge is finally transferred from the buffer gas Ne(2) (+) ion not to Kr(2) (+) but to heteronuclear NeKr(+) ion.
Experiments at the GARPUN KrF laser facility and 2D simulations using the NUTCY code were performed to study the irradiation of metal and polymethyl methacrylate (PMMA) targets by 100 ns UV pulses at intensities up to 5 × 1012 W cm−2. In both targets, a deep crater of length 1 mm was produced owing to the 2D geometry of the supersonic propagation of the ablation front in condensed matter that was pushed sideways by a conical shock wave. Small-scale filamentation of the laser beam caused by thermal self-focusing of radiation in the crater-confined plasma was evidenced by the presence of a microcrater relief on the bottom of the main crater. In translucent PMMA, with a penetration depth for UV light of several hundred micrometers, a long narrow channel of length 1 mm and diameter 30 μm was observed emerging from the crater vertex. Similar channels with a length-to-diameter aspect ratio of ∼1000 were produced by a repeated-pulse KrF laser in PMMA and fused silica glass at an intensity of ∼109 W cm−2. This channel formation is attributed to the effects of radiation self-focusing in the plasma and Kerr self-focusing in a partially transparent target material after shallow-angle reflection by the crater wall. Experimental modeling of the initial stage of inertial confinement fusion-scale direct-drive KrF laser interaction with subcritical coronal plasmas from spherical and cone-type targets using crater-confined plasmas seems to be feasible with increased laser intensity above 1014 W cm−2.
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