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Attribute measurement techniques for confirmation of declared irradiated fuel inventories at nuclear installations under safeguards surveillance are being investigated. High-gain measurements of the intensity of the Cerenkov glow from exposed assemblies in water-filled storage ponds are promising for this purpose. Such measurements have been made of Materials Testing Reactor plate-type fuel assemblies and Pressurized Water Reactor pin-type fuel assemblies. The measured intensities depend on cooling times as calculations predict. *Such was our experience in interpreting results of thermoluminescent dosimeter (TLD) measurements of the Omega West Reactor fuel elements made at the same time as the Cerenkov measurements. TLD results will be included in a separate report.

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A verification station has been designed to confirm the presence of plutonium within a container module. These container modules [about 13 cm (5 in.) in diameter and 23 cm (9 in.) high] hold sealed food-pack cans containing either plutonium oxide or metal and were designed by Sandia Laboratories to provide security and continuous surveillance and safety. After the plutonium is placed in the container module, it is closed with a solder seal. The verification station discussed here is used to confirm the presence of plutonium in the container module before it is placed in a carousel-type storage array inside the plutonium storage vault. This measurement represents the only technique that uses nuclear detectors in the plutonium protection system.