We demonstrate site-resolved imaging of a strongly correlated quantum system
without relying on laser-cooling techniques during fluorescence imaging. We
observed the formation of Mott shells in the insulating regime and realized
thermometry on the atomic cloud. This work proves the feasibility of the
noncooled approach and opens the door to extending the detection technology to
new atomic species.Comment: 5 pages, 4 figure
Engineering the thermal conductivity of amorphous materials is highly essential for the thermal management of future electronic devices. Here, we demonstrate the impact of ultrafine nanostructuring on the thermal conductivity reduction of amorphous silicon nitride (a-Si3N4) thin films, in which the thermal transport is inherently impeded by the atomic disorders. Ultrafine nanostructuring with feature sizes below 20 nm allows us to fully suppress contribution of the propagating vibrational modes (propagons), leaving only the diffusive vibrational modes (diffusons) to contribute to thermal transport in a-Si3N4. A combination of the phonon-gas kinetics model and the Allen-Feldmann theory reproduced the measured results without any fitting parameters. The thermal conductivity reduction was explained as extremely strong diffusive boundary scattering of both propagons and diffusons. These findings give rise to substantial tunability of thermal conductivity of amorphous materials, which enables us to provide better thermal solutions in microelectronic devices.
Studies
have demonstrated that the thermal conductivity (κ)
of crystalline semiconductor materials can be reduced by phonon scattering
in periodic nanostructures formed using templates fabricated from
self-assembled block copolymers (BCPs). Compared to crystalline materials,
the heat transport mechanisms in amorphous inorganic materials differ
significantly and have been explored far less extensively. However,
thermal management of amorphous inorganic solids is crucial for a
broad range of semiconductor devices. Here we present the fabrication
of freestanding amorphous silicon nitride (SiN
x
) membranes for studying κ in an amorphous solid. To
form a periodic nanostructure, directed self-assembly of cylinder-forming
BCPs is used to pattern in the SiN
x
highly
ordered, hexagonally close packed nanopores with pitch and neck width
down to 37.5 and 12 nm, respectively. The κ of the nanoporous
SiN
x
membranes is 60% smaller than the
classically predicted value based on just the membrane porosity. In
comparison, holes with much larger neck widths and pitches patterned
by e-beam lithography lead to only a slight reduction in κ,
which is closer to the classical porosity-based prediction. These
results demonstrate that κ of amorphous SiN
x
can be reduced by introducing periodic nanostructures that
behave as a phononic crystal, where the relationship between the smallest
dimension of the nanostructure and the length scale of the mean-free
paths of the dominant, heat-carrying phonons is critical. Additionally,
changing the orientation of the hexagonal array of nanopores relative
to the primary direction of heat flow has a smaller impact on amorphous
SiN
x
than was previously observed in silicon.
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