Abstract. The regional uncertainty of the column-averaged dry air mole fraction of CO2 (XCO2) retrieved using different algorithms from the Greenhouse gases Observing SATellite (GOSAT) and its attribution are still not well understood. This paper investigates the regional performance of XCO2 within a latitude band of 37–42° N segmented into 8 cells in a grid of 5° from west to east (80–120° E) in China, where typical land surface types and geographic conditions exist. The former includes desert, grassland and built-up areas mixed with cropland; and the latter includes anthropogenic emissions that change from small to large from west to east, including those from the megacity of Beijing. For these specific cells, we evaluate the regional uncertainty of GOSAT XCO2 retrievals by quantifying and attributing the consistency of XCO2 retrievals from four algorithms (ACOS, NIES, OCFP and SRFP) by intercomparison. These retrievals are then specifically compared with simulated XCO2 from the high-resolution nested model in East Asia of the Goddard Earth Observing System 3-D chemical transport model (GEOS-Chem). We also introduce the anthropogenic CO2 emissions data generated from the investigation of surface emitting point sources that was conducted by the Ministry of Environmental Protection of China to GEOS-Chem simulations of XCO2 over the Chinese mainland. The results indicate that (1) regionally, the four algorithms demonstrate smaller absolute biases of 0.7–1.1 ppm in eastern cells, which are covered by built-up areas mixed with cropland with intensive anthropogenic emissions, than those in the western desert cells (1.0–1.6 ppm) with a high-brightness surface from the pairwise comparison results of XCO2 retrievals. (2) Compared with XCO2 simulated by GEOS-Chem (GEOS-XCO2), the XCO2 values from ACOS and SRFP have better agreement, while values from OCFP are the least consistent with GEOS-XCO2. (3) Viewing attributions of XCO2 in the spatio-temporal pattern, ACOS and SRFP demonstrate similar patterns, while OCFP is largely different from the others. In conclusion, the discrepancy in the four algorithms is the smallest in eastern cells in the study area, where the megacity of Beijing is located and where there are strong anthropogenic CO2 emissions, which implies that XCO2 from satellite observations could be reliably applied in the assessment of atmospheric CO2 enhancements induced by anthropogenic CO2 emissions. The large inconsistency among the four algorithms presented in western deserts which displays a high albedo and dust aerosols, moreover, demonstrates that further improvement is still necessary in such regions, even though many algorithms have endeavored to minimize the effects of aerosols scattering and surface albedo.
Using measurements of the column-averaged CO 2 dry air mole fraction (XCO 2 ) from GOSAT and biosphere parameters, including normalized difference vegetation index (NDVI), enhanced vegetation index (EVI), leaf area index (LAI), gross primary production (GPP), and land surface temperature (LST) from MODIS, this study proposes a data-driven approach to assess the impacts of terrestrial biosphere activities on the seasonal cycle pattern of XCO 2 . A unique global land mapping dataset of XCO 2 with a resolution of 1 • by 1 • in space, and three days in time, from June 2009 to May 2014, which facilitates the assessment at a fine scale, is first produced from GOSAT XCO 2 retrievals. We then conduct a statistical fitting method to obtain the global map of seasonal cycle amplitudes (SCA) of XCO 2 and NDVI, and implement correlation analyses of seasonal variation between XCO 2 and the vegetation parameters. As a result, the spatial distribution of XCO 2 SCA decreases globally with latitude from north to south, which is in good agreement with that of simulated XCO 2 from CarbonTracker. The spatial pattern of XCO 2 SCA corresponds well to the vegetation seasonal activity revealed by NDVI, with a strong correlation coefficient of 0.74 in the northern hemisphere (NH). Some hotspots in the subtropical areas, including Northern India (with SCA of 8.68 ± 0.49 ppm on average) and Central Africa (with SCA of 8.33 ± 0.25 ppm on average), shown by satellite measurements, but missed by model simulations, demonstrate the advantage of satellites in observing the biosphere-atmosphere interactions at local scales. Results from correlation analyses between XCO 2 and NDVI, EVI, LAI, or GPP show a consistent spatial distribution, and NDVI and EVI have stronger negative correlations over all latitudes. This may suggest that NDVI and EVI can be better vegetation parameters in characterizing the seasonal variations of XCO 2 and its driving terrestrial biosphere activities. We, furthermore, present the global distribution of phase lags of XCO 2 compared to NDVI in seasonal variation, which, to our knowledge, is the first such map derived from a completely data-driven approach using satellite observations. The impact of retrieval error of GOSAT data on the mapping data, especially over high-latitude areas, is further discussed. Results from this study provide reference for better understanding the distribution of the strength of carbon sink by terrestrial ecosystems and utilizing remote sensing data in assessing the impact of biosphere-atmosphere interactions on the seasonal cycle pattern of atmospheric CO 2 columns.
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