229 Th is the only known nucleus with an excited state that offers the possibility for a direct laser excitation using existing laser technology. Its excitation energy has been measured indirectly to be 7.8(5) eV (≈160 nm). The energy and lifetime of the isomeric state make it the presently only suitable candidate for a nuclear optical clock, the uncertainty of the excitation energy is, however, still too large to allow for a direct laser excitation in a Paul trap. Therefore, a major goal during the past years has been an improved energy determination. One possible approach is to measure the kinetic energy of electrons which are emitted in the internal conversion decay of the first isomeric state in 229 Th. For this reason an electron spectrometer based on a magnetic bottle combined with electrical retarding fields has been built. Its design, as well as first test measurements are presented, which reveal a relative energy resolution of 3 % and thus enable to measure the electrons' expected kinetic energy to better than 0.1 eV. This is sufficiently precise to specify a laser system able to drive the nuclear clock transition in 229 Th.
229 Th is the only nucleus currently under investigation for the development of a nuclear optical clock (NOC) of ultra-high accuracy. The insufficient knowledge of the first nuclear excitation energy of 229 Th has so far hindered direct nuclear laser spectroscopy of thorium ions and thus the development of a NOC. Here, a nuclear laser excitation scheme is detailed, which makes use of thorium atoms instead of ions. This concept, besides potentially leading to the first nuclear laser spectroscopy, would determine the isomeric energy to 40 µeV resolution, corresponding to 10 GHz, which is a 10 4 times improvement compared to the current best energy constraint. This would determine the nuclear isomeric energy to a sufficient accuracy to allow for nuclear laser spectroscopy of individual thorium ions in a Paul trap and thus the development of a single-ion nuclear optical clock.
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