The light-matter interaction length in monolayer transition metal dichalcogenides (TMD) [1,2] on planar substrates is restricted to sub-nanometers due to their miniscule thickness. Atomically thin transition metal dichalcogenides are highly promising for integrated optoelectronic and photonic systems due to their exciton-driven linear and nonlinear interactions with light. Integrating them into optical fibers yields novel opportunities in optical communication, remote sensing, and all-fiber optoelectronics. However, the scalable and reproducible deposition of high-quality monolayers on optical fibers is a challenge. Here, the chemical vapor deposition of monolayer MoS 2 and WS 2 crystals on the core of microstructured exposed-core optical fibers and their interaction with the fibers' guided modes are reported. Two distinct application possibilities of 2D-functionalized waveguides to exemplify their potential are demonstrated. First, the excitonic 2D material photoluminescence is simultaneously excited and collected with the fiber modes, opening a novel route to remote sensing. Then it is shown that third-harmonic generation is modified by the highly localized nonlinear polarization of the monolayers, yielding a new avenue to tailor nonlinear optical processes in fibers. It is anticipated that the results may lead to significant advances in optical-fiber-based technologies.

We present a common pulse retrieval algorithm (COPRA) that can be used for a broad category of ultrashort laser pulse measurement schemes including frequency-resolved optical gating (FROG), interferometric FROG, dispersion scan, time domain ptychography, and pulse shaper assisted techniques such as multiphoton intrapulse interference phase scan (MIIPS). We demonstrate its properties in comprehensive numerical tests and show that it is fast, reliable and accurate in the presence of Gaussian noise. For FROG it outperforms retrieval algorithms based on generalized projections and ptychography. Furthermore, we discuss the pulse retrieval problem as a nonlinear least-squares problem and demonstrate the importance of obtaining a least-squares solution for noisy data. These results improve and extend the possibilities of numerical pulse retrieval. COPRA is faster and provides more accurate results in comparison to existing retrieval algorithms. Furthermore, it enables full pulse retrieval from measurements for which no retrieval algorithm was known before, e.g., MIIPS measurements. arXiv:1810.04780v1 [physics.ins-det]This document provides supplementary information to "Common pulse retrieval algorithm: a fast and universal method to retrieve ultrashort pulses". It shows additional results and contains additional information that facilitates the re-implementation of COPRA, e.g., the expressions for the gradients used in the main paper. Additionally, we provide information on the creation of the test pulses and the removal of ambiguities to facilitate the reproduction of our results.

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In this work, we demonstrate a discrete dispersion scan scheme using a low number of flat windows to vary the dispersion of laser pulses in discrete steps. Monte Carlo simulations indicate that the pulse duration can be retrieved accurately with less than 10 dispersion steps, which we verify experimentally by measuring few-cycle pulses and material dispersion curves at 3 and 10 µm wavelength. This minimal measuring scheme using only five optical components without the need for linear positioners and interferometric alignment can be readily implemented in many wavelength ranges and situations.

Active stereovision systems for the 3D measurement of surfaces rely on the sequential projection of different fringe patterns onto the scene to robustly and accurately generate 3D surface data. This limits the temporal resolution to the time by which a sufficiently high number of patterns can be projected and recorded. By encoding patterns spectrally and recording them with a hyperspectral imager, it is possible to record several patterns in a single image, limiting the temporal resolution to only the duration of the illumination. A picosecond 3D surface measurement was demonstrated using a high pulse energy femtosecond Ti:Sa laser, spectrally broadened in a hollow core fiber, and two hyperspectral cameras recording the patterns generated by diffraction at an Echelle grating.