We report on the generation of extreme ultraviolet radiation utilizing the plasmonic field enhancement in arrays of bow-tie gold optical antennae. Furthermore, their suitability to support high-order harmonic generation is examined by means of finite-difference time-domain calculations and experiments. Particular emphasis is paid to the thermal properties, which become significant at the employed peak intensities. A damage threshold depending on the antenna length is predicted and confirmed by our experimental findings. Moreover, the gas density in the vicinity of the antennae is characterized experimentally to determine the number of atoms contributing to the measured radiation, which is almost an order of magnitude larger than previously reported.
We report on low-order harmonic generation utilising the plasmonic field enhancement in arrays of rodtype gold optical antennae. Furthermore, we examine their suitability to support high-order harmonic generation (HHG). The low-order harmonics are used as a tool to investigate the nonlinear properties of the antennae. Particular attention is paid to the thermal properties, which become significant at the peak intensities necessary for HHG. A theoretical model explains the experimental findings and enables future improvements. In experiments we observe up to the fifth harmonic order and measure a field enhancement sufficient to support high-order harmonic generation. Moreover, we find a damage threshold for the antennae.
Following the impact of a single femtosecond light pulse on nickel nanostripes, material deformations-or "nanobumps"-are created. We have studied the dependence of these nanobumps on the length of nanostripes and verified the link with plasmons. More specifically, local electric currents can melt the nanostructures in the hotspots, where hydrodynamic processes give rise to nanobumps. This process is further confirmed by independently simulating local magnetic fields, since these are produced by the same local electric currents.
High-order harmonic generation in xenon with oscillator repetition rates is studied. The necessary intensity is reached via plasmonic field enhancement at nanostructured arrays of bow-tie gold antennae. The theoretical analysis focuses on the thermal properties and the damage threshold of the bow-tie antennae. On the experimental side the number of contributing atoms is determined and optimized. Extreme ultraviolet radiation is successfully observed with photon fluxes almost an order of magnitude larger than previously reported.
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