Hybrids plasmonic nanoparticles (NPs) and unique 2D graphene significantly enhanced the photoresponse of the photodetectors. The metallic NPs that exhibit localized surface plasmon resonance (LSPR) improves strong light absorption, scattering and localized electromagnetic field by the incident photons depending on the optimum condition of NPs. We report high-performance photodetectors based on reduced graphene oxide (rGO) integrated with monometallic of Au and Ag nanoparticles via a familiar fabrication technique using an electron beam evaporation machine. Under 680 nm illumination of light, our rGO photodetector exhibited the highest performance for Au-rGO with the highest responsivity of 67.46 AW−1 and the highest specific detectivity (2.39 × 1013 Jones). Meanwhile, Ag-rGO achieved the highest responsivity of 17.23 AW−1, specific detectivity (7.17 × 1011 Jones) at 785 nm. The response time are 0.146 µs and 0.135 µs for Au-rGO and Ag-rGO respectively for both wavelengths. The proposed photodetector with combining monometallic and graphene provide a new strategy to construct reliable and next-generation optoelectronic devices at VIS–NIR region.
This research focuses on the side-polished Single-Mode Optical Fibers (SMOF) as refractive index (RI) sensor utilizing properties of Surface Plasmon Resonance. The SMOF with cladding stripped off shows a D-shaped optical fiber with high sensitivity functionalization. Here we show silver protected by graphene oxide (GO) as viable candidates. A few layers of GO on top of silver thin layer were applied as a material to overcome silver coating degradation process. This silver/GO sensor was characterized using various RIs of analyte likely deionized water and alcohol solutions. Sensor with GO has shown fast response and high sensitivity in respect of RI, where sensitivity increases in range from 1.30 to 1.34 RIU (refractive index unit). This device shows highest sensitivity of up to 833.33 nm/ RIU. The polishing process using SMOF stops at few microns above the core of the fiber with the drop of output power fixed to be 1 dB as an indication to standardize the amount of cladding been removed. The thickness of 30 nm Ag was deposited using electron beam evaporation method on D-shaped optical fiber with subsequent protected layer of GO in solutions form. The use of COMSOL Multiphysics has also been carried out to observe numerical findings. The response of the GO has shown a sensitivity improvement which proves new promising approaches for the newly developed sensors.
To coordinate the resonant wavelength of the plasmonic nanoparticles (NPs), the emission band of the reduced graphene oxide (rGO) photodetector at the NIR-region is crucial for the optimal plasmon-enhanced luminescence in the device. In contrast to monometallic NPs, where limits the dimensions and extended resonant wavelength, we integrated an Au-Ag bimetallic NPs (BMNPs) to enable resonance tuning at the longer wavelength at the excitation source of 785 nm. These features showed an increase in radiative recombination rates as well as the quantum yield efficiency of the device. The BMNPs were produced from the dewetting process of 600 °C and 500 °C, both at 1 min after the deposition thickness layer of Au (8 nm) and Ag (10 nm) on the Si substrate using the electron-beam evaporation process. Our BMNPs-rGO photodetector exhibited the responsivity of 2.25 · A W−1, Jones of specific detectivity of 2.45×1011Jones, and external quantum efficiency (EQE) of 356%. The rise time and fall time for the photodetector were 32 ns and 186 ns, respectively. This work provided an essential information to enable the versatile plasmon-enhanced application in 2-dimensional (2D) material optoelectronic devices.
scite is a Brooklyn-based organization that helps researchers better discover and understand research articles through Smart Citations–citations that display the context of the citation and describe whether the article provides supporting or contrasting evidence. scite is used by students and researchers from around the world and is funded in part by the National Science Foundation and the National Institute on Drug Abuse of the National Institutes of Health.