Land use, air pollution, and climate change are closely related. This article analysed the contributions of urban land use to ambient air quality in Bahir Dar and Hawassa cities. A total of 32 geo-referenced locations, 16 each in Bahir Dar and Hawassa, representing different land uses, were assessed for carbon monoxide (CO), carbon dioxide (CO 2 ), and volatile organic compound (VOC). CO 2 concentration (ppm) for Bahir Dar and Hawassa ranged from 385.10 ± 15.34 ppm (recreational land use) to 555.50 ± 80.79 ppm (commercial land use) and 388.07 ± 19.79 ppm (recreational land use) to 444.50 ± 54.05 ppm (industrial land use), respectively, whereas mean concentration of CO was 0.01 ± 0.01 ppm (recreational land use) to 2.59 ± 0.69 ppm (circulation land use) and 0.12 ± 0.11 ppm (recreational land use) to 4.66 ± 1.41 ppm (circulation land use), respectively. The VOC values were 882.10 ± 147.05 ppm (residential land use) to 1436.00 ± 932.06 ppm (institutional land use) and 1377.30 ± 233.23 ppm (institutional land use) to 2132.33 ± 739.71 ppm (circulation land use). Inadequate monitoring, occasioned by dearth of equipment, poor urban management strategy, fossil fuel combustion, and aged vehicles were some of the factors responsible for the observed concentrations. Elevated levels of CO, CO 2 , and VOC in the atmosphere have a significant impact on global warming, with adverse effects on human health. Capacity for monitoring, analysis, reporting, and validation of air quality data in the cities should be strengthened.
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