The optical response of nonparabolic quantum wells is dominated by a strong peak at the plasmon frequency. When the electrons reach the anharmonic regions, resonant absorption becomes inefficient. This limitation is overcome by using a chirped laser pulse in the autoresonant regime. By direct simulations using the Wigner phase-space approach, we prove that, with a sequence of just a few pulses, electrons can be efficiently detrapped from a nonparabolic well. For an array of multiple quantum wells, we can create and control an electronic current by suitably applying an autoresonant laser pulse and a slowly varying dc electric field.
We present multiply differential cross sections for electron-impact ionization of the water molecule. The experimental results are compared with theoretical cross sections calculated using a recently developed distorted-wave Born approach for molecules. The experimental cross sections exhibit a very large recoil scattering, which is not predicted by the theory. This has implications for applications of this theoretical approach in areas such as modeling of ionization in biological systems.
We present a combined experimental and theoretical study of fragmentation of small Cn clusters (n = 5,7,9) produced in charge transfer collisions of fast (nu = 2.6 a.u.) singly charged Cn+ clusters with He. Branching ratios for all possible fragmentation channels have been measured. Comparison with microcanonical Metropolis Monte Carlo simulations based on quantum chemistry calculations allows us to determine the energy distribution of the excited clusters just after the collision.
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