Laser pulse irradiation of the globular turbostratic carbon material in various conditions was carried out in this work. It was investigated by TEM that the formation of nanostructured particles (nanocapsules) during irradiation at 1064 nm wavelength occurs with power density of 108 W/cm2, and it’s rise up to 1011 W/cm2 leads to increase the degree of ordering of the obtained structures. It is shown that irradiation of the initial globules with pulses at 532 nm wavelength allows to reduce the interplanar spacing of graphene layers from 0,410 nm to 0,346 nm in the formed nanocapsules. The dependence of the maximum heating temperature of nanoparticles on the energy density on the laser spot was analyzed. The influence of the heating temperature of the carbon nanomaterial on structure and morphology was stated.