A lidar system has been built to measure atmospheric-density fluctuations and the temperature in the upper stratosphere, the mesosphere, and the lower thermosphere, measurements that are important for an understanding of climate and weather phenomena. This lidar system, the Purple Crow Lidar, uses two transmitter beams to obtain atmospheric returns resulting from Rayleigh scattering and sodium-resonance fluorescence. The Rayleigh-scatter transmitter is a Nd:YAG laser that generates 600 mJ/pulse at the second-harmonic frequency, with a 20-Hz pulse-repetition rate. The sodium-resonance-fluorescence transmitter is a Nd:YAG-pumped ring dye laser with a sufficiently narrow bandwidth to measure the line shape of the sodium D(2) line. The receiver is a 2.65-m-diameter liquid-mercury mirror. A container holding the mercury is spun at 10 rpm to produce a parabolic surface of high quality and reflectivity. Test results are presented which demonstrate that the mirror behaves like a conventional glass mirror of the same size. With this mirror, the lidar system's performance is within 10% of theoretical expectations. Furthermore, the liquid mirror has proved itself reliable over a wide range of environmental conditions. The use of such a large mirror presented several engineering challenges involving the passage of light through the system and detector linearity, both of which are critical for accurate retrieval of atmospheric temperatures. These issues and their associated uncertainties are documented in detail. It is shown that the Rayleigh-scatter lidar system can reliably and routinely measure atmospheric-density fluctuations and temperatures at high temporal and spatial resolutions.

Stratospheric ozone attenuates harmful ultraviolet radiation and protects the Earth's biosphere. Ozone is also of fundamental importance for the chemistry of the lowermost part of the atmosphere, the troposphere. At ground level, ozone is an important by-product of anthropogenic pollution, damaging forests and crops, and negatively affecting human health. Ozone is critical to the chemical and thermal balance of the troposphere because, via the formation of hydroxyl radicals, it controls the capacity of tropospheric air to oxidize and remove other pollutants. Moreover, ozone is an important greenhouse gas, particularly in the upper troposphere. Although photochemistry in the lower troposphere is the major source of tropospheric ozone, the stratosphere-troposphere transport of ozone is important to the overall climatology, budget and long-term trends of tropospheric ozone. Stratospheric intrusion events, however, are still poorly understood. Here we introduce the use of modern windprofiler radars to assist in such transport investigations. By hourly monitoring the radar-derived tropopause height in combination with a series of frequent ozonesonde balloon launches, we find numerous intrusions of ozone from the stratosphere into the troposphere in southeastern Canada. On some occasions, ozone is dispersed at altitudes of two to four kilometres, but on other occasions it reaches the ground, where it can dominate the ozone density variability. We observe rapid changes in radar tropopause height immediately preceding these intrusion events. Such changes therefore serve as a valuable diagnostic for the occurrence of ozone intrusion events. Our studies emphasize the impact that stratospheric ozone can have on tropospheric ozone, and show that windprofiler data can be used to infer the possibility of ozone intrusions, as well as better represent tropopause motions in association with stratosphere-troposphere transport.

Abstract. An ensemble of space-borne and ground-based instruments has been used to evaluate the quality of the version 2.2 temperature retrievals from the Atmospheric Chemistry Experiment Fourier Transform Spectrometer (ACE-FTS). The agreement of ACE-FTS temperatures with other sensors is typically better than 2 K in the stratosphere and upper troposphere and 5 K in the lower mesosphere. There is evidence of a systematic high bias (roughly 3-6 K) in the ACE-FTS temperatures in the mesosphere, and a possible systematic low bias (roughly 2 K) in ACE-FTS temperatures near 23 km. Some ACE-FTS temperature profiles exhibit unphysical oscillations, a problem fixed in preliminary comparisons with temperatures derived using the next version of the ACE-FTS retrieval software. Though these relatively large oscillations in temperature can be on the order of 10 K in the mesosphere, retrieved volume mixing ratio profiles typically vary by less than a percent or so. Statistical comparisons suggest these oscillations occur in about 10% of the retrieved profiles. Analysis from a set of coincident lidar measurements suggests that the random error in ACE-FTS version 2.2 temperatures has a lower limit of about ±2 K.

Abstract.Temperature measurements from the PCL Rayleigh lidar located near London, Canada, taken during the 11 year period from 1994 to 2004 are used to form a temperature climatology of the middle atmosphere. A unique feature of the PCL temperature climatology is that it extends from 35 to 95 km allowing comparison with other Rayleigh lidar climatologies (which typically extend up to about 85 km), as well as with climatologies derived from sodium lidar measurements which extend from 83 to 108 km. The derived temperature climatology is compared to the CIRA-86 climatological model and to other lidar climatologies, both Rayleigh and sodium. The PCL climatology agrees well with the climatologies of other Rayleigh lidars from similar latitudes, and like these other climatologies shows significant differences from the CIRA-86 temperatures in the mesosphere and lower thermosphere. Significant disagreement is also found between the PCL climatology and sodium lidar climatologies measured in the central and western United States at similar latitudes, with the PCL climatology consistently 10 to 15 K cooler in the 85 to 90 km region.

A new method is introduced that allows meteor radars to potentially produce height-dependent temperatures, rather than simply averages over the meteor region. The method is applied to data from the Clovar radar, near London, Ontario, and then a three-way comparison between Rayleigh lidar temperatures, hydroxyl temperatures, and meteor temperatures is undertaken. The three methods prove to be complementary. The OH measurements have good accuracy, but suffer slightly from lack of precise knowledge about their height and the fact that they are effectively integrated over the depth of the OH layer. The lidar temperatures are measured at well-defined altitudes and have better accuracy than the meteor method. The meteor temperatures have the largest errors, but still provide sufficient accuracy for many types of atmospheric studies, and have the advantage that these measurements can be made 24 h a day and in all sky conditions (including during cloud and strong sunlight and moonlight). The measurements from these instruments are complementary in that they are useful for studying the temperature on different time and altitude scales. PACS No.: 94.10.Dy