Circularly polarized light is incident on a nanostructured chiral meta‐surface. In the nanostructured unit cells whose chirality matches that of light, superchiral light is forming and strong optical second harmonic generation can be observed.
Abstract:While it has been demonstrated that, above its resolution limit, Second Harmonic Generation (SHG) microscopy can map chiral local field enhancements, below that limit, structural defects were found to play a major role. Here we show that, even below the resolution limit, the contributions from chiral local field enhancements to the SHG signal can dominate over those by structural defects. We report highly homogeneous SHG micrographs of star-shaped gold nanostructures, where the SHG circular dichroism effect is clearly visible from virtually every single nanostructure. Most likely, size and geometry determine the dominant contributions to the SHG signal in nanostructured systems.
References and links1. J. B. Pendry, "A chiral route to negative refraction," Science 306(5700), 1353-1355 (2004 1983-1986 (1983). 7. T. Petralli-Mallow, T. M. Wong, J. D. Byers, H. I. Yee, and J. M. Hicks, "Circular dichroism spectroscopy at interfaces: a surface second harmonic generation study," J. Phys. Chem. 97(7), 1383-1388 (1993). 8. P. Fischer and F. Hache, "Nonlinear optical spectroscopy of chiral molecules," Chirality 17(8), 421-437 (2005).
We have performed transport measurements on bridges patterned in misaligned thin films of the superconductor Tl2Ba2CaCu2O8. There is a c-axis component of current flow along the bridge, giving rise to hysteretic Josephson-like current–voltage curves. The temperature dependence of the critical current follows the Ambegaokar–Baratoff theory with IcRN up to 26 mV at 4.2 K. Microwave emission from the Josephson junctions near Tc (≈103 K) has been detected using an X-band detector. We show that 700±15 junctions in the bridge are actively oscillating, confirming that the junctions are “intrinsic” junctions formed by adjacent copper oxide planes in the Tl2Ba2CaCu2O8 crystal structure.
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