We report on spectroscopy study of elementary magnetic excitations in an Ising-like antiferromagnetic chain compound SrCo2V2O8 as a function of temperature and applied transverse magnetic field up to 25 T. An optical as well as an acoustic branch of confined spinons, the elementary excitations at zero field, are identified in the antiferromagnetic phase below the Néel temperature of 5 K and described by a one-dimensional Schrödinger equation. The confinement can be suppressed by an applied transverse field and a quantum disordered phase is induced at 7 T. In this disordered paramagnetic phase, we observe three emergent fermionic excitations with different transverse-field dependencies. The nature of these modes is clarified by studying spin dynamic structure factor of a 1D transverse-field Heisenberg-Ising (XXZ) model using the method of infinite time evolving block decimation. Our work reveals emergent quantum phenomena and provides a concrete system for testifying theoretical predications of one-dimension quantum spin models.
We report a systematic study of low-energy lattice vibrations in the layered systems KY(MoO), KDy(MoO), KEr(MoO), and KTm(MoO). A layered crystal structure and low symmetry of the local environment of the rare-earth ion cause the appearance of vibrational and electronic excitations in Terahertz frequencies. The interaction between these excitations leads to sophisticated dynamical properties, including non-linear effects in paramagnetic resonance spectra. The THz study in magnetic field allows for the clear distinction between lattice vibrations and electronic excitations. We measured the THz transmission spectra and show that the low energy lattice vibrations in binary molybdates can be well described within the quasi-one-dimensional model. The developed model describes the measured far-infrared spectra, and results of our calculations agree with previous Raman and ultrasound studies.
Electron paramagnetic resonance spectra of KTm(MoO 4 ) 2 were measured as a function of magnetic field between 3 and 11.5 cm −1 at T = 2 K. We found that in addition to the absorption line caused by the electronic excitation of Tm 3+ ions, the spectra contain sidebands. Far-infrared transmission measured with polarized light from 10 to 75 cm −1 revealed vibration modes at 16.7 and 25.7 cm −1 for polarizations E ω a and E ω c, respectively. We show that sidebands in the spectra of paramagnetic resonance result from a parametric resonance between the electronic excitations of the Tm 3+ ions and the acoustic vibrations of the crystal lattice.
The ac magnetoconductance of bulk InSb at THz frequencies in high magnetic fields, as measured by the transmission of THz radiation, shows a field-induced transmission, which at high temperatures (≈100 K) is well explained with classical magnetoplasma effects (helicon waves). However, at low temperatures (4 K), the transmitted radiation intensity shows magnetoquantum oscillations that represent the Shubnikov-de Haas effect at THz frequencies. At frequencies above 0.9 THz, when the radiation period is shorter than the Drude scattering time, an anomalously high transmission is observed in the magnetic quantum limit that can be interpreted as carrier localization at high frequencies.
We report the observation of cyclotron resonance (CR) transitions of holes in the magnetotransmission spectra of gallium-doped germanium at low temperatures, using intense, pulsed THz free-electron laser radiation with a photon energy lower than the ionization energy of the Ga dopants (11 meV). The THz radiation, in the range of 12-89 cm −1 , both creates free holes through photoionization of Ga and induces the CR of these holes. For photon energies above the lowest energy internal Ga transition (55 cm −1 ), intradopant transitions are simultaneously observed with narrow CR peaks. For energies below 55 cm −1 , with increasing THz radiation intensity first the lowest Landau level transitions of all heavy-hole and light-hole subbands appear. This marks the onset of photoionization, which is found to be more efficient for lower laser frequencies, consistent with field-ionization (Keldysh parameter << 1). For the highest laser intensities, the CR peaks of the heavy (light) holes shift to higher (lower) magnetic field, as a result of the increasing population of the higher-energy nonequidistant Landau levels, consistent with the effective-mass theory of the hole subbands in Ge.
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