The lignite long-lasting exploitation has resulted in a series of negative impacts on the air quality of the lignite basin of Ptolemaida, Amynteo and Florina. The coal-fired plants in this region are the greatest sources of air pollutants, such as SO2, NOX, CO2, PM, heavy metals and fly ash. In this study, we investigate the air quality of Western Macedonia based on measurements of PM2.5 and PM10 in ten air quality monitoring stations (Filotas, Koilada, Oikismos, Petrana, Komi, Amyntaio, Florina, Vevi-Meliti, Pontokomi and Anargyroi) which are located in the broader area of the lignite power plants. The trends of PM time series over a 12-year period (2010-2021) show a gradual decrease of PM2.5 and PM10 concentrations following the decline of lignite production in Greece. In order to characterize the underlying atmospheric and anthropogenic processes affecting the PM concentrations we assessed the ratios of PM2.5 to PM10. The high ratios of PM2.5/PM10 indicate a major contribution of fine particles attributable to anthropogenic air pollution sources, while small ratios indicate that coarse particles are dominant, which might be related to natural sources of air pollution. We found that average PM2.5/PM10 ratios during the study period ranged between 0.48 in Oikismos and 0.70 in Florina and Vevi-Meliti. For Florina and Vevi-Meliti, the daily PM2.5/PM10 ratios were found to reach the value of 1.0, while the daily average ratios of PM2.5/PM10 were above 0.9 for almost the 15 % of the days in these sites. In the other sites high daily ratios of PM2.5/PM10 were found for a lesser number of days. The high ratios which have been found at these sites indicate the considerable contribution of energy combustion for heating purposes and other anthropogenic processes. Overall, we used the PM2.5/PM10 ratio to characterize the processes affecting the air quality within the local environment.

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Western Macedonia, located in North-western Greece, is largely dominated by lignite mining and lignite-fired power plants, which are a significant part of the country’s economy. However, the electricity generation and the related activities are among the greatest sources of air pollutants. In this study, we focus on the air quality of Western Macedonia based on measurements of Particulate Matter (PM2.5 and PM10) over a 12-year period (from 2010 to 2021) and a sampling of PM-bound trace elements over the course of 12 months (from December 2017 to November 2018). The analysis revealed an overall decrease of PM2.5 and PM10 concentrations over the study period. In general, the concentrations of PM exhibited seasonality patterns associated with the weather conditions and the local sources of air pollutants. These major sources of air pollution are the lignite mining processes, the emissions from the lignite-fired power plants, and the anthropogenic emissions from the biomass burning and heating systems. In addition, the analysis of the PM-bound trace elements revealed some differences; the elemental profiles of both PM2.5 and PM10 were quite similar, while the most abundant elements (Ca and Si) indicate that the main emission sources were related with the mining activities and the coal combustion.