Deuterium-tritium-loaded capsules at the National Ignition Facility (NIF) are now regularly producing a neutron rich high energy density plasma (nHEDP) with a low-energy "ICF-thermal" neutron density > 10 21 neutrons/cm 3 . These low-energy neutrons are produced via multiple scatter off of the highly compressed capsule and therefore provide insight into the confinement time (τ confinement ) of the assembled plasma. Neutrons are formed in the center of the 5 m NIF chamber that is well suited for minimizing "room return" thermal capture. This nHEDP environment is befitting for activation-based measurements of the (n,γ) cross sections responsible for the formation of heavy elements in astrophysical settings. These experiments also offer the first opportunity to search for the effects of nuclear-plasma interaction-induced excited state population on (n,x) reaction rates in a stellar-like plasma environment. Unfortunately, no capability currently exists at the NIF to measure the neutron spectrum in a capsule down to the 100 eV level required to enable these new classes of nuclearplasma experiments. In this paper we will discuss nHEDP-based neutron capture experiments, compare them to accelerator-based (n,γ) measurements, and discuss the requirements for a NIF-based low energy neutron spectrometer (LENS).
Indirect laser-induced fluorescence was used for the detection of several lanthanide species separated by capillary electrophoresis. Quinine sulfate was the fluorescent component of the background electrolyte, and α-hydroxyisobutyric acid was added as a complexing agent to enable the separation of analyte ions that have similar mobilities. The UV lines (333-364 nm) of an argon ion laser were used as the excitation source with a diode array detector for monitoring the fluorescent emission at 442 nm. Electrokinetic injections and transient isotachophoresis were implemented to stack the analyte ions into more concentrated zones. On-line preconcentration factors were determined to be ∼700 and resulted in limits of detection for La(3+), Ce(3+), Pr(3+), Nd(3+), Sm(3+), and Eu(3+) in the low-ppb range (6-11 nM).
We describe a radiochemical measurement of the ratio of isotope concentrations produced in a gold hohlraum surrounding an Inertial Confinement Fusion capsule at the National Ignition Facility (NIF). We relate the ratio of the concentrations of (n,γ) and (n,2n) products in the gold hohlraum matrix to the down-scatter of neutrons in the compressed fuel and, consequently, to the fuel's areal density. The observed ratio of the concentrations of (198m+g)Au and (196g)Au is a performance signature of ablator areal density and the fuel assembly confinement time. We identify the measurement of nuclear cross sections of astrophysical importance as a potential application of the neutrons generated at the NIF.
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