A strongly tilted, nearly axisymmetric vortex in dry air with asymmetric diabatic heating is analysed here by matched asymptotic expansions. The vortex is in gradient wind balance, with vortex Rossby numbers of order unity, and embedded in a quasigeostrophic (QG) background wind with weak vertical shear. With wind speeds of 60-120 km h −1, such vortices correspond to tropical storms or nascent hurricanes according to the Saffir-Simpson scale. For asymmetric heating, nonlinear coupling of the evolution equations for the vortex tilt, its core structure, and its influence on the QG background is found. The theory compares well with the established linear theory of precessing quasi-modes of atmospheric vortices, and it corroborates the relationship between vortex tilt and asymmetric potential temperature and vertical velocity patterns as found by Jones (Q. J. R. Meteorol. Soc., vol. 121, 1995, pp. 821-851) and Frank & Ritchie (Mon. Weath. Rev., vol. 127, 1999, pp. 2044-2061 in simulations of adiabatic tropical cyclones. A relation between the present theory and the local induction approximation for three-dimensional slender vortex filaments is established.

Abstract. Homogeneous freezing of solution droplets is an important pathway of ice formation in the tropopause region. The nucleation rate can be parameterized as a function of water activity, based on empirical fits and some assumptions on the underlying properties of super-cooled water, although a general theory is missing. It is not clear how nucleation events are influenced by the exact formulation of the nucleation rate or even their inherent uncertainty. In this study we investigate the formulation of the nucleation rate of homogeneous freezing of solution droplets (1) to link the formulation to the nucleation rate of pure water droplets, (2) to derive a robust and simple formulation of the nucleation rate, and (3) to determine the impact of variations in the formulation on nucleation events. The nucleation rate can be adjusted, and the formulation can be simplified to a threshold description. We use a state-of-the-art bulk ice microphysics model to investigate nucleation events as driven by constant cooling rates; the key variables are the final ice crystal number concentration and the maximum supersaturation during the event. The nucleation events are sensitive to the slope of the nucleation rate but only weakly affected by changes in its absolute value. This leads to the conclusion that details of the nucleation rate are less important for simulating ice nucleation in bulk models as long as the main feature of the nucleation rate (i.e. its slope) is represented sufficiently well. The weak sensitivity of the absolute values to the nucleation rate suggests that the amount of available solution droplets also does not crucially affect nucleation events. The use of only one distinct nucleation threshold function for analysis and model parameterization should be reinvestigated, since it corresponds to a very high nucleation rate value, which is not reached in many nucleation events with low vertical updrafts. In contrast, the maximum supersaturation and thus the nucleation thresholds reached during an ice nucleation event depend on the vertical updraft velocity or cooling rate. This feature might explain some high supersaturation values during nucleation events in cloud chambers and suggests a reformulation of ice nucleation schemes used in coarse models based on a purely temperature-dependent nucleation threshold.